We present a high-power and broadband terahertz (THz) time-domain spectroscopy setup utilizing the nonlinear organic crystal MNA both as an emitter and a detector. The THz source is based on optical rectification of near-infrared laser pulses at a central wavelength of 1036 nm from a commercial, high-power Yb-based laser system and reaches a high THz average power of 11 mW at a repetition rate of 100 kHz and a broad bandwidth of more than 9 THz without a significant power fall-off in the higher THz frequency components. The conversion efficiency is high (0.13%) in spite of the high excitation average power of 8 W. We validate the high dynamic range and reliability of the source for applications in linear spectroscopy by measuring the broadband THz properties of χ(2) nonlinear crystals up to 8 THz. This new high-repetition-rate source is very promising for ultra-broadband THz spectroscopy at high dynamic range and/or reduced measurement time.

Free-space strong-field terahertz (THz) pulses, generated via optical rectification of femtosecond lasers in nonlinear crystals, are pivotal in various applications. However, conventional Ti:sapphire lasers struggle to produce high-average-power THz sources due to their limited output power. While kilowatt ytterbium lasers are increasingly adopted, their application in THz generation faces challenges: low optical-to-THz conversion efficiency (attributed to long pulse duration and low energy) and crystal damage under high pumping power. Here, we report a high-average-power strong-field THz source using a lithium niobate crystal pumped by a 1030 nm, 570 fs, 1 mJ, 50 kHz ytterbium femtosecond laser with tilted pulse front pumping (TPFP). By systematically optimizing TPFP implementations and comparing grating- and echelon-type configurations, we achieve a THz source with 64.5 mW average power at 42 W, 50 kHz pumping, and focused peak electric field of 525 kV/cm at 0.83 mJ, 1 kHz operation. Additionally, we observe Zeeman torque signals in cobalt-iron ferromagnetic nanofilms. This high-repetition-rate, high-average-power THz system, combined with its potential capabilities in high signal-to-noise ratio spectroscopy and imaging, promises transformative impacts in quantum matter manipulation, non-destructive testing, and biomedicine.

We report the first demonstration of high-efficiency ultraviolet (UV) pulse generation in a resonance-free anti-resonant hollow-core fiber (AR-HCF). Using the wet-etching technique, we successfully reduced the cladding-tube wall thickness of the AR-HCF to 115 nm, thereby eliminating all cladding-induced structural resonances between the near-infrared pump and the deep UV wavelengths. This structural modification fundamentally suppresses competing conversion to other phase-matching points induced by structural resonances and mitigates the pump spectral broadening limitation, achieving a UV conversion efficiency as high as 12%—twice that of previous demonstrations in gas-filled AR-HCFs. This UV conversion efficiency is comparable to that of meter-scale gas-filled capillaries that require pump pulse energy of hundreds of microjoules while also maintaining the AR-HCF’s inherent advantages of centimeter-scale compactness and low pump energy at the few microjoule level.

Lithium tetraborate (LB4) is a lithium borate compound known for its exceptional linear and nonlinear optical properties, including a wide transparency range (0.16–3.5 μm) and high Raman gain. Here, a millimeter-sized LB4 whispering gallery mode (WGM) resonator with a record quality factor of 2.0×109 at 517 nm was fabricated using single-point diamond cutting. Pumped with about 10 mW at 517 nm, it demonstrated four cascaded stimulated Raman scattering (SRS) peaks (537–608 nm), with the first-order SRS achieving a threshold of 0.71 mW and 7.2% slope efficiency. To our knowledge, this marks the first LB4 WGM resonator Raman laser.

A tightly synchronized fiber laser system composed of two mode-locked Yb-doped fiber lasers in a master-slave configuration is built. The synchronization could sustain for more than 6 h, and the maximum tolerance of cavity length mismatch is measured to be about 210 μm. Afterward, a time-stretch dispersive Fourier transform technique is introduced to analyze the synchronization process over multiple cycles. The pulse evolution, center wavelength shift, spectral reshaping, and broadening are all clearly detected. And the synchronization time is experimentally determined on the order of microseconds (hundreds of roundtrips). These results also show the seed pulse acting as a temporal gate for mode locking in some cases. To the best of our knowledge, this is the first time that pulse formation, spectral evolution, center wavelength shift, and synchronization time during the synchronization process are precisely revealed in experiment. These results would help to improve the performances of synchronized laser devices and deeply understand the mechanisms of the synchronization process and other light-light interactions in materials.

The rapid growth of deep learning applications has sparked a revolution in computing paradigms, with optical neural networks (ONNs) emerging as a promising platform for achieving ultra-high computing power and energy efficiency. Despite great progress in analog optical computing, the lack of scalable optical nonlinearities and losses in photonic devices pose considerable challenges for power levels, energy efficiency, and signal latency. Here, we report an end-to-end all-optical nonlinear activator that utilizes the energy conversion of Brillouin scattering to perform efficient nonlinear processing. The activator exhibits an ultra-low activation threshold (24 nW), a wide transmission bandwidth (over 40 GHz), strong robustness, and high energy transfer efficiency. These advantages provide a feasible solution to overcome the existing bottlenecks in ONNs. As a proof-of-concept, a series of tasks is designed to validate the capability of the proposed activator as an activation unit for ONNs. Simulations show that the experiment-based nonlinear model outperforms classical activation functions in classification (97.64% accuracy for MNIST and 87.84% for Fashion-MNIST) and regression (with a symbol error rate as low as 0%) tasks. This work provides valuable insights into the innovative design of all-optical neural networks.

An object or system is said to be chiral if it cannot be superimposed on its mirror reflection. Chirality is ubiquitous in nature, for example, in protein molecules and chiral phonons—acoustic waves carrying angular momentum—which are usually either intrinsically present or magnetically excited in suitable materials. Here, we report the use of intervortex forward Brillouin scattering to optically excite chiral flexural phonons in a twisted photonic crystal fiber, which is itself a chiral material capable of robustly preserving circularly polarized optical vortex states. The phonons induce a spatiotemporal rotating linear birefringence that acts back on the optical vortex modes, coupling them together. We demonstrate intervortex frequency conversion under the mediation of chiral flexural phonons and show that, for the same phonons, backward and forward intervortex conversion occurs at different wavelengths. The results open up, to our knowledge, new perspectives for Brillouin scattering and the chiral flexural phonons offer new opportunities for vortex-related information processing and multi-dimensional vectorial optical sensing.

Submicron-thick thin-film lithium niobate (TFLN) has emerged as a promising platform for nonlinear integrated photonics. In this work, we demonstrate the efficient simultaneous generation of broadband 2nd–8th harmonics in chirped periodically poled (CPP) TFLN. This is achieved through the synergistic effects of cascaded χ(2) nonlinear up-conversion and χ(3) self-phase modulation, driven by near-infrared femtosecond pulses with a central wavelength of 2100 nm and a pulse energy of 1.2 μJ. Remarkably, the 7th and 8th harmonics extend into the deep ultraviolet (DUV) region, reaching wavelengths as short as 250 nm. The 3rd–8th harmonic spectra seamlessly connect, forming a broadband supercontinuum spanning from the DUV to the visible range (250–800 nm, -25 dB), with an on-chip conversion efficiency of 19% (0.23 μJ). This achievement is attributed to the CPP-TFLN providing multiple broadband reciprocal lattice vector bands, enabling quasi-phase matching for a series of χ(2) nonlinear processes, including second harmonic generation (SHG), cascaded SHG, and third harmonic generation. Furthermore, we demonstrated the significant role of cascaded χ(2) phase-mismatched nonlinear processes in high-harmonic generation (HHG). Our work unveils the intricate and diverse nonlinear optical interactions in TFLN, offering a clear path toward efficient on-chip HHG and compact coherent white-light sources extending into the DUV.

Femtosecond laser filamentation has attracted significant attention due to its applications in remote sensing of atmospheric pollutants and artificial weather intervention. Nitrogen is the most abundant gas in the atmosphere, and its stimulated ultraviolet emission is remarkably clean, distinctly different from the fluorescence obtained through electron impact or laser breakdown. While numerous experiments and mechanism analyses have been conducted on its characteristic fluorescence excited by laser filamentation, they predominantly focused on short-distance filamentation (less than 1 m). Contrary to previous reports, we find that at long distances (30 m), the fluorescence intensity of neutral nitrogen molecules excited by linearly polarized laser pulses is approximately 7 times that excited by circularly polarized pulses with the same energy. This enhancement is caused by the enhanced tunneling ionization rate, 3.7 times that under circular polarization, and the elongated filament length, 1.85 times that under circular polarization, when using linear polarization. Additionally, after comparing existing theories for N2(C3Πu)) excitation, the dissociation-recombination model is found to be more appropriate for explaining the formation of N2(C3Πu)) excited states during long-distance filamentation.

Simultaneously increasing the spectral bandwidth and average output power of mid-infrared supercontinuum sources remains a major challenge for their practical application. We particularly address this issue for the long mid-infrared spectral region through experimental developments of short tapered rods made from selenide glass by means of supercontinuum generation in the femtosecond regime. Our simple post-processing of glass rods unlocks potentially higher-power and coherent fiber-based supercontinuum sources beyond the 10-μm waveband. By using a 5-cm-long tapered Ge-Se-Te rod pumped at 6 μm, a supercontinuum spanning from 2 to 15 μm (3–14 μm) with an average output power of 93 mW (170 mW) is obtained for 500-kHz (1-MHz) repetition rate. Additional experiments on other glass families (silica and tellurite) covering distinct spectral regions are also reported to develop and support our analyses. We demonstrate that ultra-broadband spectral broadenings over entire glass transmission windows can be achieved in few-cm-long segments of tapered rods by a fine adjustment of input modal excitation. Numerical simulations are used to confirm the main contribution of the fundamental mode in the ultrafast nonlinear dynamics, as well as the possible preservation of coherence features. Our study opens a new route, to our knowledge, towards the power scaling of high-repetition-rate fiber supercontinuum sources over the full molecular fingerprint region.

With the rapid development of the Internet of Things and big data, integrated optical switches are gaining prominence for applications in on-chip optical computing, optical memories, and optical communications. Here, we propose a novel approach for on-chip optical switches by utilizing the nonlinear optical Kerr effect induced spontaneous symmetry breaking (SSB), which leads to two distinct states of counterpropagating light in ring resonators. This technique is based on our first experimental observation of on-chip symmetry breaking in a high-Q (9.4×106) silicon nitride resonator with a measured SSB threshold power of approximately 3.9 mW. We further explore the influence of varying pump powers and frequency detunings on the performance of SSB-induced optical switches. Our work provides insights into the development of new types of photonic data processing devices and provides an innovative approach for the future implementation of on-chip optical memories.

Laser diodes are widely used and play a crucial role in myriad modern applications including nonlinear optics and photonics. Here, we explore the four-wave mixing effect in a laser diode gain medium induced by the feedback from the high-Q microring resonator. This phenomenon can be observed at a laser frequency scan close to the microresonator eigenfrequency, prior to the transition of the laser diode from a free-running to a self-injection locking regime. The effect opens up the possibility for generation of remarkably low-noise, stable, and adjustable microwave signals. We provide a detailed numerical study of this phenomenon proven with experimental results and demonstrate the generation of the signals in the GHz range. The obtained results reveal the stability of such regime and disclose the parameter ranges enabling to achieve it. Cumulatively, our findings uncover, to our knowledge, a novel laser diode operation regime and pave the way for the creation of new types of chip-scale, low-noise microwave sources, which are highly demanded for diverse applications, including telecommunication, metrology, and sensing.

Image reconstruction through the opaque medium has great significance in fields of biophotonics, optical imaging, mesoscopic physics, and optical communications. Previous researches are limited in the simple linear scattering process. Here, we develop a nonlinear speckle decoder network, which can reconstruct the phase information of the fundamental frequency wave via the nonlinear scattering signal. Further, we validate the ability of our model to recover simple and complex structures by using MNIST and CIFAR data sets, respectively. We then show that the model is able to restore the image information through different sets of nonlinear diffusers and reconstruct the image of a kind of completely unseen object category. The proposed method paves the way to nonlinear scattering imaging and information encryption.

Thin-film periodically poled lithium niobate (TF-PPLN) devices have recently gained prominence for efficient wavelength conversion processes in both classical and quantum applications. However, the patterning and poling of TF-PPLN devices today are mostly performed at chip scales, presenting a significant bottleneck for future large-scale nonlinear photonic systems that require the integration of multiple nonlinear components with consistent performance and low cost. Here, we take a pivotal step towards this goal by developing a wafer-scale TF-PPLN nonlinear photonic platform, leveraging ultraviolet stepper lithography and an automated poling process. To address the inhomogeneous broadening of the quasi-phase matching (QPM) spectrum induced by film thickness variations across the wafer, we propose and demonstrate segmented thermal optic tuning modules that can precisely adjust and align the QPM peak wavelengths in each section. Using the segmented micro-heaters, we show the successful realignment of inhomogeneously broadened multi-peak QPM spectra with up to 57% enhancement of conversion efficiency. We achieve a high normalized conversion efficiency of 3802% W-1 cm-2 in a 6 mm long PPLN waveguide, recovering 84% of the theoretically predicted efficiency in this device. The advanced fabrication techniques and segmented tuning architectures presented herein pave the way for wafer-scale integration of complex functional nonlinear photonic circuits with applications in quantum information processing, precision sensing and metrology, and low-noise-figure optical signal amplification.

Single-photon laser ranging has widespread applications in remote sensing and target recognition. However, highly sensitive light detection and ranging (lidar) has long been restricted in the visible or near-infrared bands. An appealing quest is to extend the operation wavelength into the mid-infrared (MIR) region, which calls for an infrared photon-counting system at high detection sensitivity and precise temporal resolution. Here, we devise and demonstrate an MIR upconversion lidar based on nonlinear asynchronous optical sampling. Specifically, the infrared probe is interrogated in a nonlinear crystal by a train of pump pulses at a slightly different repetition rate, which favors temporal optical scanning at a picosecond timing resolution and a kilohertz refreshing rate over ∼50 ns. Moreover, the cross-correlation upconversion trace is temporally stretched by a factor of 2×104, which can thus be recorded by a low-bandwidth silicon detector. In combination with the time-correlated photon-counting technique, the achieved effective resolution is about two orders of magnitude better than the timing jitter of the detector itself, which facilitates a ranging precision of 4 μm under a low detected flux of 8×10-5 photons per pulse. The presented MIR time-of-flight range finder is featured with single-photon sensitivity and high positioning resolution, which would be particularly useful in infrared sensing and imaging in photon-starved scenarios.

Vectorial beams have attracted great interest due to their broad applications in optical micromanipulation, optical imaging, optical micromachining, and optical communication. Nonlinear frequency conversion is an effective technique to expand the frequency range of the vectorial beams. However, the scheme of existing methods to generate vector beams of the second harmonic (SH) lacks compactness in the experiment. Here, we introduce a new way to realize the generation of vector beams of SH by using a nonlinear fork grating to solve such a problem. We examine the properties of generated SH vector beams by using Stokes parameters, which agree well with theoretical predictions. Then we demonstrate that linearly polarized vector beams with arbitrary topological charge can be achieved by adjusting the optical axis direction of the half-wave plate (HWP). Finally, we measure the nonlinear conversion efficiency of such a method. The proposed method provides a new way to generate vector beams of SH by using a microstructure of nonlinear crystal, which may also be applied in other nonlinear processes and promote all-optical waveband applications of such vector beams.

We present a detailed theoretical and numerical analysis on the temporal-spectral-spatial evolution of a high-peak-power femtosecond laser pulse in two sets of systems: a pure lithium niobate (LN) plate and a periodically poled lithium niobate (PPLN) plate. We develop a modified unidimensional pulse propagation model that considers all the prominent linear and nonlinear processes and carried out the simulation process based on an improved split-step Fourier transformation method. We theoretically analyze the synergic action of the linear dispersion effect, the second-order nonlinearity (2nd-NL) second-harmonic generation (SHG) effect, and the third-order nonlinearity (3rd-NL) self-phase modulation (SPM) effect, and clarify the physical mechanism underlying the peculiar and diverse spectral broadening patterns previously reported in LN and PPLN thin plate experiments. Such analysis and discussion provides a deeper insight into the synergetic contribution of these linear and nonlinear effects brought about by the interaction of a femtosecond laser pulse with the LN nonlinear crystal and helps to draw a picture to fully understand these fruitful optical physical processes, phenomena, and laws.

Polarization holography has been extensively applied in many fields, such as optical science, metrology, and biochemistry, due to its property of polarization modulation. However, the modulated polarization state of diffracted light corresponds strictly to that of incident light one by one. Here, a kind of tunable polarization holographic grating has been designed in terms of Jones matrices, and intensity-based polarization manipulation has been realized experimentally. The proposed tunable polarization holographic grating is recorded on an azobenzene liquid-crystalline film by a pair of coherent light beams with orthogonal polarization states and asymmetrically controlled intensities. It is found that the diffracted light can be actively manipulated from linearly to circularly polarized based on the light intensity of the recording holographic field when the polarization state of incident light keeps constant. Our work could enrich the field of light manipulation and holography.

Since the emergence of graphene, transition metal dichalcogenides, and black phosphorus, two-dimensional materials have attracted significant attention and have driven the development of fundamental physics and optoelectronic devices. Metal phosphorus trichalcogenides (MPX3), due to their large bandgap of 1.3–3.5 eV, enable the extension of optoelectronic applications to visible and ultraviolet (UV) wavelengths. Micro-Z/I-scan (μ-Z/I-scan) and micro-pump-probe (μ-pump-probe) setups were used to systematically investigate the third-order nonlinear optical properties and ultrafast carrier dynamics of the representative material AgInP2S6. UV-visible absorption spectra and density functional theory (DFT) calculations revealed a quantum confinement effect, in which the bandgap decreased with increasing thickness. The two-photon absorption (TPA) effect is exhibited under the excitation of both 520 and 1040 nm femtosecond pulses, where the TPA coefficient decreases as the AgInP2S6 thickness increases. In contrast, the TPA saturation intensity exhibits the opposite behavior that the TPA saturation is more likely to occur under visible excitation. After the valence band electrons undergo photon transitions to the conduction band, the non-equilibrium carriers relax through non-radiative and defect-assisted recombination. These findings provide a comprehensive understanding of the optical response process of AgInP2S6 and are a valuable reference for the development of optoelectronic devices.

Cnoidal waves are a type of nonlinear periodic wave solutions of the nonlinear dynamic equations. They are well known in fluid dynamics, but it is not the case in optics. In this paper we show both experimentally and numerically that cnoidal waves could be formed in a fiber laser either in the net normal or net anomalous cavity dispersion regime, especially because, as the pump power is increased, the formed cnoidal waves could eventually evolve into a train of bright (in the net anomalous cavity dispersion regime) or dark (in the net normal cavity dispersion regime) solitons. Numerical simulations of the laser operation based on the extended nonlinear Schrödinger equation (NLSE) have well reproduced the experimental observations. The result not only explains why solitons can still be formed in a fiber laser even without mode locking but also suggests a new effective way of automatic stable periodic pulse train generation in lasers with a nonlinear cavity.

Optical clock networks have distinct advantages for the dissemination of time/frequency, geodesy, and fundamental research. To realize such a network, the telecom band and optical atomic clocks have to be coherently bridged. Since the telecom band and optical atomic clocks reside in a distinct spectral region, second-harmonic generation is usually introduced to bridge the large frequency gap. In this paper, we introduce a new method to coherently link a 1550 nm continuous wave laser with a Ti:sapphire mode-locked laser-based optical frequency comb. By coupling the 1550 nm continuous wave laser light and the Ti:sapphire comb light together into a photonic crystal fiber, nonlinear interaction takes place, and new comblike frequency components related to the 1550 nm laser frequency are generated in the visible region. Consequently, we can detect beat notes between two combs in the visible region with a signal-to-noise ratio of more than 40 dB in a resolution bandwidth of 300 kHz. With this signal, we realize an optical frequency divider for converting the frequency of optical clocks in the visible region to the telecom band at 1.55 μm. An out-of-loop measurement shows that the additional noise and uncertainty induced in optical frequency conversion are 5×10-18 at 1 s averaging time and 2.2×10-19, respectively, which are limited by the uncompensated light path fluctuation but fulfill precision measurement using state-of-the-art optical clocks.

Nonlinear effects in microresonators are efficient building blocks for all-optical computing and telecom systems. With the latest advances in microfabrication, coupled microresonators are used in a rapidly growing number of applications. In this work, we investigate the coupling between twin-resonators in the presence of Kerr nonlinearity. We use an experimental setup with controllable coupling between two high-Q resonators and discuss the effects caused by the simultaneous presence of linear and nonlinear coupling between the optical fields. Linear-coupling-induced mode splitting is observed at low input powers, with the controllable coupling leading to a tunable mode splitting. At high input powers, the hybridized resonances show spontaneous symmetry breaking (SSB) effects, in which the optical power is unevenly distributed between the resonators. Our experimental results are supported by a detailed theoretical model of nonlinear twin-resonators. With the recent interest in coupled resonator systems for neuromorphic computing, quantum systems, and optical frequency comb generation, our work provides important insights into the behavior of these systems at high circulating powers.

This review describes recent theoretical and experimental advances in the area of multimode solitons, focusing primarily on multimode fibers. We begin by introducing the basic concepts such as the spatial modes supported by a multimode fiber and the coupled mode equations for describing the different group delays and nonlinear properties of these modes. We review several analytic approaches used to understand the formation of multimode solitons, including those based on the 3D+1 spatiotemporal nonlinear Schrödinger equation (NLSE) and its approximate 1D+1 representation that has been found to be highly efficient for studying the self-imaging phenomena in graded-index multimode fibers. An innovative Gaussian quadrature approach is used for faster numerical simulations of the 3D+1 NLSE. The impact of linear mode coupling is discussed in a separate section using a generalized Jones formalism because of its relevance to space-division multiplexed optical communication systems. The last section is devoted to the relevant experimental studies involving multimode solitons.

The trans-spectral manipulation of spatio-temporal structured light, characterized by dynamic inhomogeneous trajectories and a unique nature in the space–time domain, opens myriad possibilities for high-dimensional optical communication in the ultraviolet band. Here, we experimentally demonstrate the high-performance transfer of the spatio-temporal optical Ferris wheel beam from near-infrared to blue–violet wavelengths. Owing to the energy conservation and momentum conservation mechanism, the 420 nm output signal beam accurately retains the spatio-temporal characteristics of the 776 nm input probe optical Ferris wheel beam, facilitated by the 780 nm Gaussian pump beam. The identical multi-petal intensity profiles confirm the successful transfer of spatial characteristics from the input probe to the output signal beams. The fully synchronized rotation velocities and directions of the probe and signal beams demonstrate the precise transfer of temporal characteristics, achieving approximately 98% conversion accuracy. This work enables efficient information transfer across different wavelength bands and offers a promising approach for achieving high-dimensional quantum communication.

A Brillouin-assisted 80-GHz-spaced dual-comb source with a reconfigurable repetition frequency difference ranging from 48 MHz to 1.486 GHz is demonstrated. Two pairs of dual-pump seeds with an interval offset produce the corresponding dual Brillouin lasers in two fiber loops, and then the Brillouin lasers give rise to dual combs via the cavity-enhanced cascaded four-wave mixing effect. The repetition frequency difference is determined by the interval offset of the dual-pump seeds, which is induced by the Brillouin frequency shift difference between different fibers in a frequency shifter. Each comb provides 22 lasing lines, and the central 10 lines in a 20-dB power deviation feature high optical signal-to-noise ratios exceeding 50 dB. The linewidths of the dual-comb beating signals are less than 300 Hz, and the absolute linewidths of the comb lines are around 1.5 kHz. The dual-comb source enables substantial repetition frequency differences from 48 MHz to 1.486 GHz by changing the pluggable fibers in the frequency shifter.

Within optical microresonators, the Kerr interaction of photons can lead to symmetry breaking of optical modes. In a ring resonator, this leads to the interesting effect that light preferably circulates in one direction or in one polarization state. Applications of this effect range from chip-integrated optical diodes to nonlinear polarization controllers and optical gyroscopes. In this work, we study Kerr-nonlinearity-induced symmetry breaking of light states in coupled resonator optical waveguides (CROWs). We discover, to our knowledge, a new type of controllable symmetry breaking that leads to emerging patterns of dark and bright resonators within the chains. Beyond stationary symmetry broken states, we observe Kerr-effect-induced homogeneous periodic oscillations, switching, and chaotic fluctuations of circulating powers in the resonators. Our findings are of interest for controlled multiplexing of light in photonic integrated circuits, neuromorphic computing, topological photonics, and soliton frequency combs in coupled resonators.

Optical nonlinear response and its dynamics of wide-bandgap materials are key to realizing integrated nonlinear photonics and photonic circuit applications. However, those applications are severely limited by the unavailability of both dispersion and dynamics of nonlinear refraction (NLR) via conventional measurements. In this work, the broadband NLR dynamics with extremely high sensitivity (λ/1000) can be obtained from absorption spectroscopy in GaN:C using the refraction-related interference model. Both the absorption and refraction kinetics are found to be significantly modulated by the C-related defects. Especially, we demonstrate that the refractive index change Δn of GaN:C is negative and can be used to realize all-optical switching applications owing to the large NLR and ultrafast switching time. The NLR under different non-equilibrium carrier distributions originates from the capture of electrons by CN+ defect state, while the absorption modulation originates from the excitation of tri-carbon defects. We believe that this work provides a better understanding of the GaN:C nonlinear properties and an effective solution to broadband NLR dynamics of transparent thin films or heterostructure materials.

Responsivity is a critical parameter for sensors utilized in industrial miniaturized sensors and biomedical implants, which is typically constrained by the size and the coupling with external reader, hindering their widespread applications in our daily life. Here, we propose a highly-responsive sensing method based on Hamiltonian hopping, achieving the responsivity enhancement by 40 folds in microscale sensor detection compared to the standard method. We implement this sensing method in a nonlinear system with a pair of coupled resonators, one of which has a nonlinear gain. Surprisingly, our method surpasses the sensing performance at an exceptional point (EP)—simultaneous coalescence of both eigenvalues and eigenvectors. The responsivity of our method is notably enhanced thanks to the large frequency response at a Hamiltonian hopping point (HHP) in the strong coupling, far from the EP. Our study also reveals a linear HHP shift under different perturbations and demonstrates the detection capabilities down to sub-picofarad (<1 pF) of the microscale pressure sensors, highlighting their potential applications in biomedical implants.

A high-quality optical microcavity can enhance optical nonlinear effects by resonant recirculation, which provides a reliable platform for nonlinear optics research. When a soliton microcomb and a probe optical field are coexisting in a micro-resonator, a concomitant microcomb (CMC) induced by cross-phase modulation (XPM) will be formed synchronously. Here, we characterize the CMC comprehensively in a micro-resonator through theory, numerical simulation, and experimental verification. It is found that the CMCs spectra are modulated due to resonant radiation (RR) resulting from the interaction of dispersion and XPM effects. The group velocity dispersion induces symmetric RRs on the CMC, which leads to a symmetric spectral envelope and a dual-peak pulse in frequency and temporal domains, respectively, while the group velocity mismatch breaks the symmetry of RRs and leads to asymmetric spectral and temporal profiles. When the group velocity is linearly varying with frequency, two RR frequencies are hyperbolically distributed about the pump, and the probe light acts as one of the asymptotic lines. Our results enrich the CMC dynamics and guide microcomb design and applications such as spectral extension and dark pulse generation.

We develop a spatiotemporal mode decomposition technique to study the spatial and temporal mode power distribution of ultrashort pulses in long spans of graded-index multimode fiber, for different input laser conditions. We find that the beam mode power content in the dispersive pulse propagation regime can be described by the Bose–Einstein law, as a result of the process of power diffusion from linear and nonlinear mode coupling among nondegenerate mode groups. In the soliton regime, the output mode power distribution approaches the Rayleigh–Jeans law.

Spatial engineering of the nonlinear susceptibility χ(2) in resonant metasurfaces offers a new degree of freedom in the design of the far-field response of second-harmonic generation (SHG). We demonstrate this by applying electric field poling to lithium niobate (LN) thin films, which inverts the spontaneous polarization and thus the sign of χ(2). Metasurfaces fabricated in periodically poled LN films reveal the distinct influence of the χ(2)-patterning on the spatial distribution of the second harmonic. This work is a first step toward far-field engineering of SHG in metasurfaces with electric field poling.

Undetected-photon imaging allows for objects to be imaged in wavelength regions where traditional components are unavailable. Although first demonstrated using quantum sources, recent work has shown that the technique also holds with classical beams. To date, however, all the research in this area has exploited parametric down-conversion processes using bulk nonlinear crystals within free-space systems. Here, we demonstrate undetected-photon-based imaging using light generated via stimulated four-wave mixing within highly nonlinear silicon fiber waveguides. The silicon fibers have been tapered to have a core diameter of ∼915 nm to engineer the dispersion and reduce the insertion losses, allowing for tight mode confinement over extended lengths to achieve practical nonlinear conversion efficiencies (∼-30 dB) with modest pump powers (∼48 mW). Both amplitude and phase images are obtained using classically generated light, confirming the high degree of spatial and phase correlation of our system. The high powers (>10 nW) and long coherence lengths (>4 km) associated with our large fiber-based system result in high contrast and stable images.

Rogue waves are ubiquitous in nature, appearing in a variety of physical systems ranging from acoustics, microwave cavities, optical fibers, and resonators to plasmas, superfluids, and Bose&ndash;Einstein condensates. Unlike nonlinear solitary waves, rogue waves are extreme events that can occur even without nonlinearity by, for example, spontaneous synchronization of waves with different spatial frequencies in a linear system. Here, we report the observation of rogue-wave-like events in human red blood cell (RBC) suspensions under weak light illumination, characterized by an abnormal L-shaped probability distribution. Such biophotonic extreme events arise mostly due to the constructive interference of Mie-scattered waves from the suspended RBCs, whose biconcave shape and mutable orientation give rise to a time-dependent random phase modulation to an incident laser beam. We numerically simulate the beam propagation through the colloidal suspensions with added disorder in both spatial and temporal domains to mimic random scattering due to Brownian motion. In addition, at high power levels, nonlinear beam self-focusing is also observed, leading to a dual-exponential probability distribution associated with the formation of multiple soliton-like spots. Such rogue wave events should also exist in environments with cells of other species such as swimming bacteria, and understanding of their underlying physics may lead to unexpected biophotonic applications.

We report on the observation of conical third, fifth, seventh, and ninth harmonics that gradually emerge during the supercontinuum generation by filamentation of femtosecond midinfrared pulses in lithium strontium hexafluoroaluminate crystal. We show that the generation of conical odd harmonics is an optical signature of light-driven material reorganization in the form of volume nanogratings at the site irradiated by repetitive femtosecond filaments. The angle-resolved spectral measurements demonstrate remarkably broad spectra of individual odd harmonics, benefiting from a spectrally broadened pump pulse (supercontinuum), and reveal that filament-inscribed nanogratings represent photonic structures that are able to provide ultrabroad phase-matching bandwidths covering the wavelength range from the ultraviolet to the near infrared. We propose a scenario that interprets the generation of conical fifth, seventh, and ninth harmonics as nanograting phase-matched cascaded noncollinear four-wave mixing processes.

There are extensive studies to date on optical nonlinearities in microcavities at the near and mid-IR wavelengths. Pushing this research into the visible region is equally valuable. Here, we demonstrate a directly pumped, blue band Kerr frequency comb and stimulated Raman scattering (SRS) at 462 nm in a silica nanofiber-coupled whispering gallery microcavity system. Notably, due to the high optical intensities achieved, photodarkening is unavoidable and can quickly degrade the optical quality of both the coupling optical nanofiber and the microcavity, even at very low pump powers. Nonetheless, stable hyperparametric oscillation and SRS are demonstrated in the presence of photodarkening by taking advantage of in-situ thermal bleaching. This work highlights the challenges of silica-based, short wavelength nonlinear optics in high-quality, small mode volume devices and gives an effective method to overcome this apparent limitation, thus providing a baseline for optics research in the blue region for any optical devices fabricated from silica.

Microresonator-based optical frequency combs are broadband light sources consisting of equally spaced and coherent narrow lines, which are extremely promising for applications in molecular spectroscopy and sensing in the mid-infrared (MIR) spectral region. There are still great challenges in exploring how to improve materials for microresonator fabrication, extend spectral bandwidth of parametric combs, and realize fully stabilized soliton MIR frequency combs. Here, we present an effective scheme for broadband MIR optical frequency comb generation in a MgF2 crystalline microresonator pumped by the quantum cascade laser. The spectral evolution dynamics of the MIR Kerr frequency comb is numerically investigated, revealing the formation mechanism of the microresonator soliton comb via scanning the pump-resonance detuning. We also experimentally implement the modulation instability state MIR frequency comb generation in MgF2 resonators covering from 3380 nm to 7760 nm. This work proceeds microresonator-based comb technology toward a miniaturization MIR spectroscopic device that provides potential opportunities in many fields such as fundamental physics and metrology.

We propose a novel quantum nonlinear interferometer design that incorporates a passive parity–time (PT)-symmetric coupler sandwiched between two nonlinear sections where signal–idler photon pairs are generated. The PT symmetry enables efficient coupling of the longer-wavelength idler photons and facilitates the sensing of losses in the second waveguide exposed to analyte under investigation, whose absorption can be inferred by measuring only the signal intensity at a shorter wavelength where efficient detectors are readily available. Remarkably, we identify a new phenomenon of sharp signal intensity fringe shift at critical idler loss values, which is distinct from the previously studied PT symmetry breaking. We discuss how such unconventional properties arising from quantum interference can provide a route to enhancing the sensing of analytes and facilitate broadband spectroscopy applications in integrated photonic platforms.

By taking advantage of the optical induction method, a non-Hermitian photonic graphene lattice is efficiently established inside an atomic vapor cell under the condition of electromagnetically induced transparency. This non-Hermitian structure is accomplished by simultaneously modulating both the real and imaginary components of the refractive index into honeycomb profiles. The transmitted probe field can either exhibit a hexagonal or honeycomb intensity profile when the degree of non-Hermiticity is effectively controlled by the ratio between imaginary and real indices. The experimental realization of such an instantaneously tunable complex honeycomb potential sets a new platform for future experimental exploration of non-Hermitian topological photonics. Also, we demonstrate the Talbot effect of the transmitted probe patterns. Such a self-imaging effect based on a non-Hermitian structure provides a promising route to potentially improve the related applications, such as an all-optical-controllable Talbot–Lau interferometer.

Nonlinear Raman–Nath diffraction (NRND) offers an effective way to realize multiple noncollinear parametric processes based on the partially satisfied transverse phase-matching conditions in quadratic nonlinear media. Here, the realization of ultrabroadband NRND (UB-NRND) driven by a high-peak-power ultrashort femtosecond pump laser in two types of nonlinear crystals is reported: periodically poled lithium niobate (PPLN) and chirped PPLN (CPPLN). Multi-order ultrabroadband Raman–Nath second-harmonic (SH) signal outputs along fixed diffraction angles are simultaneously observed. This distinguished transversely phase-matched supercontinuum phenomenon is attributed to the synergic action of natural broad bandwidth of an ultrashort femtosecond pump laser and the third-order nonlinear effect induced spectral broadening, in combination with the principal ultrabroadband noncollinear second-harmonic generation processes. The NRND process with multiple quasi-phase matching (QPM) interactions from CPPLN leads to the SH output covering a wide range of wavelengths between 389 and 997 nm and exhibiting an energy conversion efficiency several orders of magnitude higher than previous studies. This UB-NRND scheme would bring better techniques and tools for applications ranging from ultrashort pulse characterization and nondestructive identification of domain structures to accurate parameter monitoring of second- and third-order nonlinear susceptibilities within solid-state nonlinear microstructured materials.

Materials with strong optical Kerr effects (OKEs) are crucial for a broad range of applications, such as all-optical data processing and quantum information. However, the underlying OKE mechanism is not clear in 2D materials. Here, we reveal key insights of the OKE associated with 2D excitons. An admirably succinct formalism is derived for predicting the spectra and the magnitude of the nonlinear refractive index (n2) of 2D materials. The predicted n2 spectra are consistent with reported experimental data and exhibit pronounced excitonic resonances, which is distinctively different from bulk semiconductors. The n2 value is predicted to be 3×10-10 cm2/W for a 2D layered perovskite at low temperature as 7 K, which is four orders of magnitude larger than those of bulk semiconductors. The superior OKE induced by 2D excitons would give rise to a narrow refractive index-near-zero region for intense laser light. Furthermore, we demonstrate that the 2D layered perovskite should exhibit the best OKE efficiency (WFOM=1.02, TFOM=0.14) at 1550 nm, meeting the material requirements for all-optical switching. Our findings deepen the understanding of the OKE of 2D semiconducting materials and pave the way for highly efficient all-optical excitonic devices.

Stimulated Brillouin scattering (SBS) has many applications; for example, in sensing, microwave photonics, and signal processing. Here, we report the first experimental study of SBS in chiral photonic crystal fiber (PCF), which displays optical activity and robustly maintains circular polarization states against external perturbations. As a result, circularly polarized pump light is cleanly backscattered into a Stokes signal with the orthogonal circular polarization state, as is required by angular momentum conservation. By comparison, untwisted PCF generates a Stokes signal with an unpredictable polarization state, owing to its high sensitivity to external perturbations. We use chiral PCF to realize a circularly polarized continuous-wave Brillouin laser. The results pave the way for a new generation of stable circularly polarized SBS systems with applications in quantum manipulation, optical tweezers, optical gyroscopes, and fiber sensors.

The high-energy few-cycle mid-infrared laser pulse beyond 2 μm is of immense importance for attosecond science and strong-field physics. However, the limited gain bandwidth of laser crystals such as Ho:YLF and Ho:YAG allows the generation of picosecond (ps) long pulses and, hence, makes it challenging to generate few-cycle pulse at 2 μm without utilizing an optical parametric chirped-pulse amplifier (OPCPA). Moreover, the exclusive use of the near-infrared wavelength has limited the generation of wavelengths beyond 4 μm (OPCPA). Furthermore, high harmonic generation (HHG) conversion efficiency reduces dramatically when driven by a long-wavelength laser. Novel schemes such as multi-color HHG have been proposed to enhance the harmonic flux. Therefore, it is highly desirable to generate few-cycle to femtosecond pulses from a 2 μm laser for driving these experiments. Here, we utilize two-stage nonlinear spectral broadening and pulse compression based on the Kagome-type hollow-core photonic crystal fiber (HC-PCF) to compress few-ps pulses to sub-50 fs from a Ho:YLF amplifier at 2 μm at 1 kHz repetition rate. We demonstrate both experimentally and numerically the compression of 3.3 ps at 140 μJ pulses to 48 fs at 11 μJ with focal intensity reaching 1013 W/cm2. Thereby, this system can be used for driving HHG in solids at 2 μm. In the first stage, the pulses are spectrally broadened in Kagome fiber and compressed in a silicon-based prism compressor to 285 fs at a pulse energy of 90 μJ. In the second stage, the 285 fs pulse is self-compressed in air-filled HC-PCF. With fine-tuning of the group delay dispersion (GDD) externally in a 3 mm window, a compressed pulse of 48 fs is achieved. This leads to a 70-fold compression of the ps pulses at 2050 nm. We further used the sub-50 fs laser pulses to generate white light by focusing the pulse into a thin medium of YAG.

We demonstrate the optomechanical cooling of a tapered optical nanofiber by coupling the polarization of light to the mechanical angular momentum of the system. The coupling is enabled by birefringence in the fiber and does not make use of an optical resonator. We find evidence for cooling in the distribution of thermally driven amplitude fluctuations and the noise spectrum of the torsional modes. Our proof-of-principle demonstration shows cavity-less cooling of the torsional degree of freedom of a macroscopically extended nanofiber.

Optical parametric oscillators (OPOs) can downconvert the pump laser to longer wavelengths with octave separation via χ(2), which is widely used for laser wavelength extension including mid-infrared (MIR) generation. Such a process can be integrated in monolithic resonators, being compact and low in threshold. In this work, we show that the monolithic χ(2) mini-OPO can also be used for optical frequency comb generation around 2096 nm and enters the boundary of MIR range. A new geometry called an optical superlattice box resonator is developed for this realization with near-material-limited quality factor of 4.0×107. Only a continuous-wave near-infrared pump laser is required, with OPO threshold of 80 mW and output power up to 340 mW. Revival temporal profiles are measured at a detectable repetition frequency of 1.426 GHz, and narrow beat note linewidth of less than 10 Hz shows high comb coherence. These results are in good agreement with our simulation for a stable comb generation. Such an OPO-based comb source is useful for carbon dioxide sensing or the mine prospect applications and can be generalized to longer MIR wavelengths for general gas spectroscopy.

Realization of the efficient steering for photons streams from nano sources is essential for further progress in integrated photonic circuits, especially when involving nonlinear sources. In general, steering for nonlinear sources needs additional optical control elements, limiting their application occasions as photonic devices. Here, we propose a simple and efficient beam steering scheme for the second-harmonic (SH) emission in the hybrid waveguide (consisting of CdSe nanobelts on the Au film) by mode-selective excitation. Adjusting the position of the incident beam illuminating on the tapered waveguide, the excitation types of guided modes can be selected, realizing the directionality control of SH emission. Stable steering of 6.1° for the SH emission is observed when the interference modes change from TE00 & TE01 to TE00 & TE02, which is confirmed by SH Fourier imaging and simulations. Our approach gets rid of the complex structural design and provides a new idea for beam steering of nonlinear optical devices with various nonlinear wavefronts.

Pursuing nanometer-scale nonlinear converters based on second harmonic generation (SHG) is a stimulating strategy for bio-sensing, on-chip optical circuits, and quantum information processing, but the light-conversion efficiency is still poor in such ultra-small dimensional nanostructures. Herein, we demonstrate a highly enhanced broadband frequency converter through a hybrid plasmonic–dielectric coupler, a ZnTe/ZnO single core–shell nanowire (NW) integrated with silver (Ag) nanoparticles (NPs). The NW dimension has been optimized to allow the engineering of dielectric resonances at both fundamental wave and second harmonic frequencies. Meanwhile, the localized surface plasmon resonances are excited in the regime between the Ag NPs and ZnTe/ZnO dielectric NW, as evidenced by plasmon-enhanced Raman scattering and resonant absorption. These two contributors remarkably enhance local fields and consequently support the strong broadband SHG outputs in this hybrid nanostructure by releasing stringent phase-matching conditions. The proposed nanoscale nonlinear optical converter enables the manipulation of nonlinear light–matter interactions toward the development of on-chip nanophotonic systems.

We report on a new method to achieve the single-scan polarization-resolved degenerate four-wave mixing (DFWM) spectroscopy in a Rb atomic medium using a vector optical field, in which two pump beams are kept linearly polarized and a vector beam is employed as the probe beam. As the polarization and intensity of the DFWM signal are closely dependent on the polarization state of the probe beam, a vector probe beam with space-variant states of polarization is able to generate a DFWM signal with space-variant states of polarization and intensity across the DFWM image. Accordingly, the polarization-resolved spectra can be retrieved from a single DFWM image. To the best of our knowledge, this is the first time that the single-scan polarization-resolved spectrum detection has been realized experimentally with a vector beam. This work provides a simple but efficient single-scan polarization-resolved spectroscopic method, which would be of great utility for the samples of poor light stability and fast optical processes.

We demonstrated an efficient scheme of measuring the angular velocity of a rotating object with the detection light working at the infrared regime. Our method benefits from the combination of second-harmonic generation (SHG) and rotational Doppler effect, i.e., frequency upconversion detection of rotational Doppler effect. In our experiment, we use one infrared light as the fundamental wave (FW) to probe the rotating objects while preparing the other FW to carry the desired superpositions of orbital angular momentum. Then these two FWs are mixed collinearly in a potassium titanyl phosphate crystal via type II phase matching, which produces the visible second-harmonic light wave. The experimental results show that both the angular velocity and geometric symmetry of rotating objects can be identified from the detected frequency-shift signals at the photon-count level. Our scheme will find potential applications in infrared monitoring.

Multimode nonlinear optics is used to overcome a long-standing limitation of fiber optics, tightly phase locking several spatial modes and enabling the coherent transport of a wave packet through a multimode fiber. A similar problem is encountered in the temporal compression of multimillijoule pulses to few-cycle duration in hollow gas-filled fibers. Scaling the fiber length to up to 6 m, hollow fibers have recently reached 1 TW of peak power. Despite the remarkable utility of the hollow fiber compressor and its widespread application, however, no analytical model exists to enable insight into the scaling behavior of maximum compressibility and peak power. Here we extend a recently introduced formalism for describing mode locking to the analog scenario of locking spatial fiber modes together. Our formalism unveils the coexistence of two soliton branches for anomalous modal dispersion and indicates the formation of stable spatiotemporal light bullets that would be unstable in free space, similar to the temporal cage solitons in mode-locking theory. Our model enables deeper understanding of the physical processes behind the formation of such light bullets and predicts the existence of multimode solitons in a much wider range of fiber types than previously considered possible.

Silicon photonic integrated devices used for nonlinear optical signal processing play a key role in ultrafast switching, computing, and modern optical communications. However, current devices suffer from limited operation speeds and low conversion efficiencies due to the intrinsically low nonlinear index of silicon. In this paper, we experimentally demonstrate enhanced optical nonlinearity in a silicon–organic hybrid slot waveguide consisting of an ultranarrow slot waveguide coated with a highly nonlinear organic material. The fabricated slot area is as narrow as 45 nm, which is, to the best of our knowledge, the narrowest slot width that has been experimentally reported in silicon slot waveguides. The nonlinear coefficient of the proposed device with a length of 3 mm is measured to be up to 1.43×106 W-1 km-1. Based on the nanostructure design, the conversion efficiencies of degenerate four-wave mixing showed enhancements of more than 12 dB and 5 dB compared to those measured for an identical device without the organic material and a silicon strip waveguide, respectively. As a proof of concept, all-optical canonical logic units based on the prepared device with two inputs at 40 Gb/s are analyzed. The obtained logic results showed clear temporal waveforms and wide-open eye diagrams with error-free performance, illustrating that our device has great potential for use in high-speed all-optical signal processing and high-performance computing in the nodes and terminals of optical networks.

Indium arsenide phosphide (InAsP) nanowires (NWs), a member of the III–V semiconductor family, have been used in various photonic and optoelectronic applications thanks to their unique electrical and optical properties such as high carrier mobility and adjustable band gap. In this work, we synthesize InAsP NWs and further explore their nonlinear optical properties. The ultrafast carrier dynamics and nonlinear optical response are thoroughly studied based on the nondegenerate pump probe and Z-scan experimental measurements. Two different characteristic carrier lifetimes (∼2 and ∼15 ps) from InAsP NWs are observed during the excited-carrier relaxation process. Based on the physical model analysis, the relaxation process can be ascribed to the carrier cooling process via carrier-phonon scattering and Auger recombination. In addition, based on the measured excited-carrier lifetime and Pauli-blocking principle, we discover that InAsP NWs show strong saturable absorption properties at the wavelengths of 532 and 1064 nm. Last, we demonstrate for the first time a femtosecond (∼426 fs) solid-state laser based on an InAsP NWs saturable absorber at 1.04 μm. We believe that our work provides a better understanding of the InAsP NWs optical properties and will further advance their photonic applications in the near-infrared range.

All-inorganic perovskite has attracted significant attention due to its excellent nonlinear optical characteristics. Stable and low-toxic perovskite materials have great application prospects in optoelectronic devices. Here, we study the nonlinear optical properties of CsPbClxBr3-x (x=1, 1.5, 2) nanocrystals (NCs) glass by open-aperture Z-scan. It is found that the two- (2PA) and three-photon absorption (3PA) intensity can be adjusted by the treatment temperature and the ratio of halide anions. The perovskite NCs glass treated at a high temperature has better crystallinity, resulting in stronger nonlinear absorption performance. In addition, the value of the 2PA parameter of CsPbCl1.5Br1.5 NCs glasses decreases when the incident pump intensity increases, which is ascribed to the saturation of 2PA and population inversion. Finally, the research results show that the 2PA coefficient (0.127 cm GW-1) and 3PA coefficient (1.21×10-5 cm3 GW-2) of CsPbCl1Br2 NCs glass with high Br anion content are larger than those of CsPbCl2Br1 and CsPbCl1.5Br1.5 NCs glasses. This is mainly due to the greater influence of Br anions on the symmetry of the perovskite structure, which leads to the redistribution of delocalized electrons. The revealed adjustable nonlinear optical properties of perovskite NCs glass are essential for developing stable and high-performance nonlinear optical devices.

Self-referenced dissipative Kerr solitons (DKSs) based on optical microresonators offer prominent characteristics allowing for various applications from precision measurement to astronomical spectrometer calibration. To date, direct octave-spanning DKS generation has been achieved only in ultrahigh-Q silicon nitride microresonators under optimized laser tuning speed or bi-directional tuning. Here we propose a simple method to easily access the octave-spanning DKS in an aluminum nitride (AlN) microresonator. In the design, two modes that belong to different families but with the same polarization are nearly degenerate and act as a pump and an auxiliary resonance, respectively. The presence of the auxiliary resonance can balance the thermal dragging effect, crucially simplifying the DKS generation with a single pump and leading to an enhanced soliton access window. We experimentally demonstrate the long-lived DKS operation with a record single-soliton step (10.4 GHz or 83 pm) and an octave-spanning bandwidth (1100–2300 nm) through adiabatic pump tuning. Our scheme also allows for direct creation of the DKS state with high probability and without elaborate wavelength or power schemes being required to stabilize the soliton behavior.

We present an experimental proposal to achieve a strong photon blockade by employing electromagnetically induced transparency (EIT) with a single alkaline-earth-metal atom trapped in an optical cavity. In the presence of optical Stark shift, both the second-order correlation function and cavity transmission exhibit asymmetric structures between the red and blue sidebands of the cavity. For a weak control field, the photon quantum statistics for the coherent transparency window (i.e., atomic quasi-dark-state resonance) are insensitive to the Stark shift, which should also be immune to the spontaneous emission of the excited state by taking advantage of the intrinsic dark-state polariton of EIT. Interestingly, by exploiting the interplay between the Stark shift and control field, the strong photon blockade at atomic quasi-dark-state resonance has an optimal second-order correlation function g(2)(0)～10-4 and a high cavity transmission simultaneously. The underlying physical mechanism is ascribed to the Stark shift enhanced spectrum anharmonicity and the EIT hosted strong nonlinearity with loss-insensitive atomic quasi-dark-state resonance, which is essentially different from the conventional proposal with emerging Kerr nonlinearity in cavity-EIT. Our results reveal a new strategy to realize high-quality single photon sources, which could open up a new avenue for engineering nonclassical quantum states in cavity quantum electrodynamics.

Nonreciprocal light propagation plays an important role in modern optical systems, from photonic networks to integrated photonics. We propose a nonreciprocal system based on a resonance-frequency-tunable cavity and intensity-adaptive feedback control. Because the feedback-induced Kerr nonlinearity in the cavity is dependent on the incident direction of light, the system exhibits nonreciprocal transmission with a transmission contrast of 0.99 and an insertion loss of 1.5 dB. By utilizing intensity-adaptive feedback control, the operating intensity range of the nonreciprocal system is broadened to 20 dB, which relaxes the limitation of the operating intensity range for nonlinear nonreciprocal systems. Our protocol paves the way to realize high-performance nonreciprocal propagation in optical systems and can also be extended to microwave systems.

We discover single and homocentric optical spheres of the three-dimensional inhomogeneous nonlinear Schr?dinger equation (NLSE) with spherical symmetry, which is a novel model of light bullets that can present a three-dimensional rogue wave. The isosurface of this light bullet oscillates along the radius direction and does not travel with the evolution of time. The localized nature of rogue wave light bullets both in space and in time, which is in complete contrast to the traveling character of the usual light bullets, is due to the localization of the rogue wave in the one-dimensional NLSE. We present also an investigation of the stability of the optical sphere solutions. The lower modes of perturbation are found to display transverse instabilities that break the spherical symmetry of the system. For the higher modes, the optical sphere solutions can be classified as stable solutions.

Brillouin spectroscopy is an important topic and powerful tool in modern optics, as the acquisitions of acoustic velocities and elastic moduli are one of the keys to investigate and analyze the contents of material science and condensed matter physics. Although stimulated Brillouin spectroscopy based on the pump-probe technique has striking advantages that include higher spectral resolution and signal-to-noise ratio, it is challenging to accomplish high-speed acquisition in the presence of pump background noise. In this paper, we propose a method for signal–noise separation through spiral phase precoding of the Brillouin spectrum signal. We achieve on-demand tailoring spatial distribution of the signal, and hence the signal can be separated from the background noise. Furthermore, this approach has little energy loss due to phase-only modulation, and retains the advantages of high efficiency and high gain in Brillouin interaction. The proof-of-principle demonstration provides a practical way to reshape the spatial structure of Brillouin spectra, and shows the potential in quasi-noise-free nonlinear interactions.

Spatial light modulators (SLMs) are devices for modulating amplitude, phase, or polarization of light beams on demand. Such devices are regarded as the backbone for optical information parallel processing and future optical computers. Currently, SLMs are mainly operated in an electrical addressing manner, wherein the optical beams are modulated by electrical signals. However, future all-optical information processing systems prefer to control light directly by light (i.e., optically addressed, OA) without electro-optical conversion. Here, we present an OASLM based on a metasurface (MS-OASLM), whose operation principle relies on nonlinear polarization control of read light by another write light at the nanoscale. Its resolution is more than 10 times higher than a typical commercial SLM and achieves 500 line pairs per millimeter (corresponding to a pixel size of only 1 μm). The MS-OASLM shows unprecedented compactness and is only 400 nm in thickness. Such MS-OASLMs could provide opportunities to develop next generation all-optical information processing and high resolution display technologies.

We demonstrate the generation of wavelength-tunable deep-ultraviolet pulses in a small-mode-area hollow-core fiber fabricated by tapering a nodeless tubular-type hollow-core fiber. Down-scaling of the cross-sectional geometry reduces the pump energy requirement for inducing sufficient nonlinear effects, presenting a unique opportunity for staging low-energy-threshold gas-based nonlinear optics. We report the onset of the ultraviolet light with the pump pulse energy as low as 125 nJ. Our numerical analysis shows that the frequency conversion arises due to soliton phase matching, and therefore shot-to-shot coherence of the ultraviolet emission is well-preserved. It offers a promising platform for a compact ultraviolet frequency comb source.

Multimode optical fibers are attracting a growing interest for their capability to transport high-power laser beams, coupled with novel nonlinear optics-based applications. However, optical fiber breakdown occurs when beam intensities exceed a certain critical value. Optical breakdown associated with irreversible modifications of the refractive index, triggered by multiphoton absorption, has been largely exploited for fiber material micro-structuration. Here we show that, for light beam intensities slightly below the breakdown threshold, nonlinear absorption strongly affects the dynamics of a propagating beam as well. We experimentally analyze this subthreshold regime and highlight the key role played by spatial self-imaging in graded-index fibers for enhancing nonlinear optical losses. We characterize the nonlinear power transmission properties of multimode fibers for femtosecond pulses propagating in the near-infrared spectral range. We show that an effective N-photon absorption analytical model is able to describe the experimental data well.

Synchronization has great impacts in various fields such as self-clocking, communication, and neural networks. Here, we present a mechanism of synchronization for two mechanical modes in two coupled optomechanical resonators with a parity-time (PT)-symmetric structure. It is shown that the degree of synchronization between the two far-off-resonant mechanical modes can be increased by decreasing the coupling strength between the two optomechanical resonators due to the large amplification of optomechanical interaction near the exceptional point. Additionally, when we consider the stochastic noises in the optomechanical resonators by working near the exceptional point, we find that more noises can enhance the degree of synchronization of the system under a particular parameter regime. Our results open up a new dimension of research for PT-symmetric systems and synchronization.

Nonlinear optical processes in waveguides play important roles in compact integrated photonics, while efficient coupling and manipulations inside the waveguides still remain challenging. In this work, we propose a new scheme for second-harmonic generation as well as beam shaping in lithium niobate slab waveguides with the assistance of well-designed grating metasurfaces at λ=1064 nm. By encoding the amplitude and phase into the holographic gratings, we further demonstrate strong functionalities of nonlinear beam shaping by the metasurface design, including dual focusing and Airy beam generation. Our approach would inspire new designs in the miniaturization and integration of compact multifunctional nonlinear light sources on chip.

The manipulation of the polarization properties of light in guided media is crucial in many classical and quantum optical systems. However, the capability of current technology to finely define the state of polarization of particular wavelengths is far from the level of maturity in amplitude control. Here, we introduce a light-by-light polarization control mechanism with wavelength selectivity based on the change of the phase retardance by means of stimulated Brillouin scattering. Experiments show that any point on the Poincaré sphere can be reached from an arbitrary input state of polarization with little variation of the signal amplitude (2.5 dB). Unlike other Brillouin processing schemes, the degradation of the noise figure is small (1.5 dB for a full 2π rotation). This all-optical polarization controller can forge the development of new polarization-based techniques in optical communication, laser engineering, sensing, quantum systems, and light-based probing of chemical and biological systems.

We report an indium phosphide nanowire (NW)-induced cavity in a silicon planar photonic crystal (PPC) waveguide to improve the light–NW coupling. The integration of NW shifts the transmission band of the PPC waveguide into the mode gap of the bare waveguide, which gives rise to a microcavity located on the NW section. Resonant modes with Q factors exceeding 103 are obtained. Leveraging on the high density of the electric field in the microcavity, the light–NW interaction is enhanced strongly for efficient nonlinear frequency conversion. Second-harmonic generation and sum-frequency generation in the NW are realized with a continuous-wave pump laser in a power level of tens of microwatts, showing a cavity-enhancement factor of 112. The hybrid integration structure of NW-PPC waveguide and the self-formed microcavity not only opens a simple strategy to effectively enhance light–NW interactions, but also provides a compact platform to construct NW-based on-chip active devices.

The reorientation of 2D materials caused by nonlocal electron coherence is the formation mechanism of 2D material spatial self-phase modulation under laser irradiation, which is widely known as the “wind-chime” model. Here, we present a method that provides strong evidence for the reorientation of 2D-material-induced spatial self-phase modulation. The traditional “wind-chime” model was modified by taking into account the attenuation, i.e., damping of the incident light beam in the direction of the optical path. Accordingly, we can extract the nonlinear refractive index of a single MoS2 nanosheet, instead of simply obtaining the index from an equivalent MoS2 film that was constructed by all nanosheets. Our approach introduces a universal and accurate method to extract intrinsic nonlinear optical parameters from 2D material systems.

We demonstrate both experimentally and theoretically the trapping and guiding of a weak signal pulse via a self-accelerating Airy pulse. This is achieved by launching the Airy pulse in the anomalous dispersion regime of an optical fiber, thereby inducing a gravity-like potential that can compel the signal pulse in the normal dispersion regime to undergo co-acceleration. Such guiding pulse by pulse can be controlled at ease simply by altering the acceleration conditions of the Airy pulse. Furthermore, the guided signal can be featured with either single or double peaks, which is explained by using the theory of fundamental and second-order quasi-modes associated with the gravity-like potential. Our work represents, to our knowledge, the first demonstration of pulse guiding in the anomalous dispersion regime of any self-accelerating pulse.

Raman lasers based on integrated silica whispering gallery mode resonant cavities have enabled numerous applications from telecommunications to biodetection. To overcome the intrinsically low Raman gain value of silica, these devices leverage their ultrahigh quality factors (Q), allowing submilliwatt stimulated Raman scattering (SRS) lasing thresholds to be achieved. A closely related nonlinear behavior to SRS is stimulated anti-Stokes Raman scattering (SARS). This nonlinear optical process combines the pump photon with the SRS photon to generate an upconverted photon. Therefore, in order to achieve SARS, the efficiency of the SRS process must be high. As a result, achieving SARS in on-chip resonant cavities has been challenging due to the low lasing efficiencies of these devices. In the present work, metal-doped ultrahigh Q (Q>107) silica microcavity arrays are fabricated on-chip. The metal-dopant plays multiple roles in improving the device performance. It increases the Raman gain of the cavity material, and it decreases the optical mode area, thus increasing the circulating intensity. As a result, these devices have SRS lasing efficiencies that are over 10× larger than conventional silica microcavities while maintaining low lasing thresholds. This combination enables SARS to be generated with submilliwatt input powers and significantly improved anti-Stokes Raman lasing efficiency.

Mid-infrared (mid-IR) imaging and spectroscopic techniques have been rapidly evolving in recent years, primarily due to a multitude of applications within diverse fields such as biomedical imaging, chemical sensing, and food quality inspection. Mid-IR upconversion detection is a promising tool for exploiting some of these applications. In this paper, various characteristics of mid-IR upconversion imaging in the femtosecond regime are investigated using a 4f imaging setup. A fraction of the 100 fs, 80 MHz output from a Ti:sapphire laser is used to synchronously pump an optical parametric oscillator, generating 200 fs mid-IR pulses tunable across the 2.7&ndash;4.0 &mu;m wavelength range. The signal-carrying mid-IR pulses are detected by upconversion with the remaining fraction of the original pump beam inside a bulk LiNbO3 crystal, generating an upconverted field in the visible/near-IR range, enabling silicon-based CCD detection. Using the same pump source for generation and detection ensures temporal overlap of pulses inside the nonlinear crystal used for upconversion, thus resulting in high conversion efficiency even in a single-pass configuration. A theory is developed to calculate relevant acceptance parameters, considering the large spectral bandwidths and the reduced interaction length due to group velocity mismatch, both associated with ultrashort pulses. Furthermore, the resolution of this ultrashort-pulsed upconversion imaging system is described. It is demonstrated that the increase in acceptance bandwidth leads to increased blurring in the upconverted images. The presented theory is consistent with experimental observations.

Mid-infrared pulsed lasers operating around the 3?μm wavelength regime are important for a wide range of applications including sensing, spectroscopy, imaging, etc. Despite the recent advances in technology, the lack of a nonlinear optical modulator operating in the mid-infrared regime remains a significant challenge. Here, we report the third-order nonlinear optical response of gold nanorods (GNRs) ranging from 800?nm to the mid-infrared regime (2810?nm) enabled by their size and overlapping behavior-dependent longitudinal surface plasmon resonance. In addition, we demonstrate a wavelength-tunable Er3+-doped fluoride fiber laser modulated by GNRs, which can deliver pulsed laser output, with the pulse duration down to 533?ns, tunable wavelength ranging from 2760.2 to 2810.0?nm, and spectral 3?dB bandwidth of about 1?nm. The experimental results not only validate the GNRs’ robust mid-infrared nonlinear optical response, but also manifest their application potential in high-performance broadband optoelectronic devices.

We present the results of research carried out for the first time, to the best of our knowledge, on the generation of terahertz radiation under the action of “single-color” and “dual-color” high-power femtosecond laser pulses on liquefied gas–liquid nitrogen. Our experimental results supported by careful theoretical interpretation showed clearly that under femtosecond laser radiation, liquid and air emit terahertz waves in a very different way. We assumed that the mobility of ions and electrons in liquid can play an essential role, forming a quasi-static electric field by means of ambipolar diffusion mechanism.

Dispersion engineering in optical waveguides allows applications relying on the precise control of phase matching conditions to be implemented. Although extremely effective over relatively narrow band spectral regions, dispersion control becomes increasingly challenging as the bandwidth of the process of interest increases. Phase matching can also be achieved by exploiting the propagation characteristics of waves exciting different spatial modes of the same waveguide. Phase matching control in this case relies on achieving very similar propagation characteristics across two, and even more, waveguide modes over the wavelengths of interest, which may be rather far from one another. We demonstrate here that broadband (>40??nm) four-wave mixing can be achieved between pump waves and a signal located in different bands of the communications spectrum (separated by 50?nm) by exploiting interband nonlinearities. Our demonstration is carried out in the silicon-rich silicon nitride material platform, which allows flexible device engineering, allowing for strong effective nonlinearity at telecommunications wavelengths without deleterious nonlinear-loss effects.

This paper describes the specially designed geometry of a dry-etched large-wedge-angle silica microdisk resonator that enables anomalous dispersion in the 780 nm wavelength regime. This anomalous dispersion occurs naturally without the use of a mode-hybridization technique to control the geometrical dispersion. By fabricating a 1-μm-thick silica microdisk with a wedge angle as large as 56° and an optical Q-factor larger than 107, we achieve a visible Kerr comb that covers the wavelength interval of 700–897 nm. The wide optical frequency range and the closeness to the clock transition at 698 nm of Sr87 atoms make our visible comb a potentially useful tool in optical atomic clock applications.

Raman and Brillouin lasers based on a high-quality (high-Q) whispering gallery mode microresonator (WGMR) are usually achieved by employing a tunable single-frequency laser as a pump source. Here, we experimentally demonstrate visible Raman and Brillouin lasers using a compact microresonator/ZrF4 BaF2 LaF3 AlF3 NaF (ZBLAN)-fiber hybrid system by incorporating a WGMR with a fiber-compatible distributed Bragg reflector/fiber Bragg grating to form a Fabry–Perot (F-P) fiber cavity and using a piece of Pr:ZBLAN fiber as gain medium. The high-Q silica-microsphere not only offers a Rayleigh-scattering-induced backreflection to form the ～635 nm red laser oscillation in the F-P fiber cavity, but also provides a nonlinear gain in the WGMR itself to generate either stimulated Raman scattering or stimulated Brillouin scattering. Up to six-order cascaded Raman lasers at 0.65 μm, 0.67 μm, 0.69 μm, 0.71 μm, 0.73 μm, and 0.76 μm are achieved, respectively. Moreover, a Brillouin laser at 635.54 nm is clearly observed. This is, to the best of our knowledge, the first demonstration of visible microresonator-based lasers created by combining a Pr:ZBLAN fiber. This structure can effectively extend the laser wavelength in the WGMR to the visible waveband and may find potential applications in underwater communication, biomedical diagnosis, microwave generation, and spectroscopy.

Two-dimensional materials are generating great interest due to their unique electrical and optical properties. In particular, transition metal dichalcogenides such as molybdenum disulfide (MoS2) are attractive materials due to the existence of a direct band gap in the monolayer limit that can be used to enhance nonlinear optical phenomena, such as Raman spectroscopy. Here, we have investigated four-wave mixing processes in bulk MoS2 using a multiplex coherent anti-Stokes Raman spectroscopy setup. The observed four-wave mixing signal has a resonance at approximately 680 nm, corresponding to the energy of the A excitonic transition of MoS2. This resonance can be attributed to the increased third-order nonlinear susceptibility at wavelengths near the excitonic transition. This phenomenon could open the path to using MoS2 as a substrate for enhancing four-wave mixing processes such as coherent anti-Stokes Raman spectroscopy.

We demonstrate a passively mode-locked all-fiber laser incorporating a piece of graded-index multimode fiber as a mode-locking modulator based on a nonlinear multimodal interference technique, which generates two types of coexisting high-energy ultrashort pulses [i.e., the conventional soliton (CS) and the stretched pulse (SP)]. The CS with pulse energy as high as 0.38 nJ is obtained at the pump level of 130 mW. When the pump increases to 175 mW, the high-energy SP occurs at a suitable nonlinear phase bias and its pulse energy can reach 4 nJ at a 610 mW pump. The pulse durations of the generated CS and SP are 2.3 ps and 387 fs, respectively. The theory of nonlinear fiber optics, single-shot spectral measurement by the dispersive Fourier-transform technique, and simulation methods based on the Ginzburg–Landau equation are provided to characterize the laser physics and reveal the underlying principles of the generated CS and SP. A rogue wave, observed between the CS and SP regions, mirrors the laser physics behind the dynamics of generating a high-energy SP from a CS. The proposed all-fiber laser is versatile, cost-effective and easy to integrate, which provides a promising solution for high-energy pulse generation.

We demonstrate a stable conventional soliton in a Tm-doped hybrid mode-locked fiber laser by employing a homemade all-fiber Lyot filter (AFLF) and a single-wall carbon nanotube. The AFLF, designed by sandwiching a piece of polarization-maintained fiber (PMF) with two 45° tilted fiber gratings inscribed by a UV laser in PMF with a phase-mask scanning technique, shows large filter depth of ～9 dB and small insertion loss of ～0.8 dB. By optimizing the free spectral range of the AFLF, the Kelly sidebands of a conventional soliton centered at 1966.4 nm can be dramatically suppressed without impairing the main shape of the soliton spectrum. It gives the pulse duration of 1.18 ps and bandwidth of 3.8 nm. By adjusting the temperature of the PMF of the AFLF from 7°C to 60°C, wavelength tunable soliton pulses ranging from 1971.62 nm to 1952.63 nm are also obtained. The generated soliton pulses can be precisely tuned between 1971.62 nm and 1952.63 nm by controlling the temperature of the AFLF.

The quantum multimode of correlated fields is essential for future quantum-correlated imaging. Here we investigate multimode properties theoretically and experimentally for the parametric amplified multiwave mixing process. The multimode behavior of the signals in our system stems from spatial phase mismatching caused by frequency resonant linewidth. In the spatial domain, we observe the emission rings with an uneven distribution of photon intensity in the parametric amplified four-wave mixing process, suggesting different spatial modes. The symmetrical distribution of spatial spots indicates the spatial correlation between the Stokes and anti-Stokes signals. While in the frequency domain, the multimode character is reflected as multiple peaks splitting in the signals’ spectrum. A novelty in our experiment, the number of multimodes both in the spatial and frequency domains can be controlled by dressing lasers by modifying the nonlinear susceptibility. Finally, we extend the multimode properties to the multiwave mixing process. The results can be applied in quantum imaging.

We present the design, fabrication, and characterization of a highly nonlinear few-mode fiber (HNL-FMF) with an intermodal nonlinear coefficient of 2.8 (W·km) 1, which to the best of our knowledge is the highest reported to date. The graded-index circular core fiber supports two mode groups (MGs) with six eigenmodes and is highly doped with germanium. This breaks the mode degeneracy within the higher-order MG, leading to different group velocities among corresponding eigenmodes. Thus, the HNL-FMF can support multiple intermodal four-wave mixing processes between the two MGs at the same time. In a proof-of-concept experiment, we demonstrate simultaneous intermodal wavelength conversions among three eigenmodes of the HNL-FMF over the C band.

We have developed a numerical framework that allows estimation of coherence in spatiotemporal and spatiospectral domains. Correlation properties of supercontinuum (SC) pulses generated in a bulk medium are investigated by means of second-order coherence theory of non-stationary fields. The analysis is based on simulations of individual space–time and space–frequency realizations of pulses emerging from a 5 mm thick sapphire plate, in the regimes of normal, zero, and anomalous group velocity dispersion. The temporal and spectral coherence properties are analyzed in the near field (as a function of spatial position at the exit plane of the nonlinear medium) and as a function of propagation direction (spatial frequency) in the far field. Unlike in fiber-generated SC, the bulk case features spectacularly high degrees of temporal and spectral coherence in both the spatial and spatial-frequency domains, with increasing degrees of coherence at higher pump energies. When operating near the SC generation threshold, the overall degrees of temporal and spectral coherence exhibit an axial dip in the spatial domain, whereas in the far field, the degree of coherence is highest around the optical axis.

Recently, the perfect vector (PV) beam has sparked considerable interest because its radius is independent of the topological charge (TC), which has demonstrated special capabilities in optical manipulation, microscopy imaging, and laser micromachining. Previous research about the generation and manipulation of such PV beams only focuses on the linear optical fields. Therefore, the generation of nonlinear PV beams is still lacking. Here, we propose a dual waveband generator to simultaneously generate the PV beams in linear and nonlinear wavebands. In our experiment, PV beams with different polarization states are realized. It is proved that the polarization states of the generated PV beams can be flexibly adjusted by changing the axis direction of a half wave plate. The experimental results show that the radii of the generated PV beams are equal and independent of the TCs. With proper alteration of the nonlinear crystals, this approach could be further extended to other nonlinear processes, such as sum-frequency generation and difference-frequency generation.

Historically, nonlinear optical phenomena such as spectral broadening by harmonic generation have been associated with crystals owing to their strong nonlinear refractive indices, which are in the range of ～10 14 cm2/W. This association was also the result of the limited optical power available from early lasers and the limited interaction length that the laser–crystal interaction architecture could offer. Consequently, these limitations disqualified a large number of materials whose nonlinear coefficient is lower than n2～10 16 cm2/W as suitable materials for nonlinear optics applications. For example, it is a common practice in most of optical laboratories to consider ambient or atmospheric air as a “nonlinear optically” inert medium due to its very low nonlinear coefficient (～10.10 19 cm2/W) and low density. Today, the wide spread of high-power ultra-short pulse lasers on one hand, and low transmission loss and high-power handling of Kagome hollow-core photonic crystal fiber on the other hand, provide the necessary ingredients to excite strong nonlinear optical effects in practically any gas media, regardless of how low its optical nonlinear response is. By using a single table-top 1 mJ ultra-short pulse laser and an air exposed inhibited-coupling guiding hollow-core photonic crystal fiber, we observed generation of supercontinuum and third harmonic generation when the laser pulse duration was set at 600 fs and Raman comb generation when the duration was 300 ps. The supercontinuum spectrum spans over ～1000 THz and exhibits a typical spectral-density energy of 150 nJ/nm. The dispersion profile of inhibited-coupling hollow-core fiber imprints a distinctive sequence in the supercontinuum generation, which is triggered by the generation of a cascade of four-wave mixing lines and concluded by solitonic dynamics. The Raman comb spans over 300 THz and exhibits multiple sidebands originating from N2 vibrational and ro-vibrational Raman transitions. With the growing use of hollow-core photonic crystal fiber in different fields, the results can be applied to mitigate air nonlinear response when it is not desired or to use ambient air as a convenient nonlinear medium.

A hybrid no-core fiber (NCF)–graded index multimode fiber (GIMF) structure is used as a saturable absorber (SA) for mode-locked laser operation. Such an SA supports various types of soliton outputs. By changing the cavity parameters, not only the spatiotemporal mode-locking states with a stable single pulse but also tightly and loosely bound solitons are generated. Single 35.5 pJ solitons centered at 1568.5 nm have a 4 nm spectral full-width at half-maximum and an 818 fs temporal duration. Tightly bound soliton pairs with continuously tunable wavelength from 1567.48 nm to 1576.20 nm, featured with an ～700 fs pulse train with a separation of 2.07 ps, have been observed by stretching the NCF-GIMF structured device. Meanwhile, several different pulse separations from 37.57 ps to 56.46 ps of loosely bound solitons have also been realized. The results provide help in understanding the nonlinear dynamics in fiber lasers.

We experimentally demonstrate self-trapping of light, as a result of plasmonic resonant optical nonlinearity, in both aqueous and organic (toluene) suspensions of gold nanorods. The threshold power for soliton formation is greatly reduced in toluene as opposed to aqueous suspensions. It is well known that the optical gradient forces are optimized at off-resonance wavelengths at which suspended particles typically exhibit a strong positive (or negative) polarizability. However, surprisingly, as we tune the wavelength of the optical beam from a continuous-wave (CW) laser, we find that the threshold power is reduced by more than threefold at the plasmonic resonance frequency. By analyzing the optical forces and torque acting on the nanorods, we show theoretically that it is possible to align the nanorods inside a soliton waveguide channel into orthogonal orientations by using merely two different laser wavelengths. We perform a series of experiments to examine the transmission of the soliton-forming beam itself, as well as the polarization transmission spectrum of a low-power probe beam guided along the soliton channel. It is found that the expected synthetic anisotropic properties are too subtle to be clearly observed, in large part due to Brownian motion of the solvent molecules and a limited ordering region where the optical field from the self-trapped beam is strong enough to overcome thermodynamic fluctuations. The ability to achieve tunable nonlinearity and nanorod orientations in colloidal nanosuspensions with low-power CW laser beams may lead to interesting applications in all-optical switching and transparent display technologies.

Interest in the nonlinear properties of multi-mode optical waveguides has seen a recent resurgence on account of the large dimensionality afforded by the platform. The large volume of modes in these waveguides provides a new spatial degree of freedom for phase matching nonlinear optical processes. However, this spatial dimension is quantized, which narrows the conversion bandwidths of intermodal processes and constrains spectral and temporal tailoring of the light. Here we show that by engineering the relative group velocity within the spatial dimension, we can tailor the phase-matching bandwidth of intermodal parametric nonlinearities. We demonstrate group-velocity-tailored parametric nonlinear mixing between higher-order modes in a multi-mode fiber with gain bandwidths that are more than an order of magnitude larger than that previously thought possible for intermodal four-wave mixing. As evidence of the technological utility of this methodology, we seed this process to generate the first high-peak-power wavelength-tunable all-fiber quasi-CW laser in the Ti:sapphire wavelength regime. More generally, with the combination of intermodal interactions, which dramatically expand the phase-matching degrees of freedom for nonlinear optics, and intermodal group-velocity engineering, which enables tailoring of the bandwidth of such interactions, we showcase a platform for nonlinear optics that can be broadband while being wavelength agnostic.

We investigate the properties of spatial solitons in the fractional Schr dinger equation (FSE) with parity-time (PT)-symmetric lattice potential supported by the focusing of Kerr nonlinearity. Both one- and two-dimensional solitons can stably propagate in PT-symmetric lattices under noise perturbations. The domains of stability for both one- and two-dimensional solitons strongly depend on the gain/loss strength of the lattice. In the spatial domain, the solitons are rigidly modulated by the lattice potential for the weak diffraction in FSE systems. In the inverse space, due to the periodicity of lattices, the spectra of solitons experience sharp peaks when the values of wavenumbers are even. The transverse power flows induced by the imaginary part of the lattice are also investigated, which can preserve the internal energy balances within the solitons.

In this work, we report the modeling and the experimental demonstration of intermodal spontaneous as well as stimulated four-wave mixing (FWM) in silicon waveguides. In intermodal FWM, the phase-matching condition is achieved by exploiting the different dispersion profiles of the optical modes in a multimode waveguide. Since both the energy and the wave vectors have to be conserved in the FWM process, this leads to a wide tunability of the generated photon wavelength, allowing us to achieve a large spectral conversion. We measured several waveguides that differ by their widths and demonstrate large signal generation spanning from the pump wavelength (1550 nm) down to 1202 nm. A suited setup evidences that the different waves propagated indeed on different order modes, which supports the modeling. Despite observing a reduced efficiency with respect to intramodal FWM due to the decreased modal overlap, we were able to show a maximum spectral distance between the signal and idler of 979.6 nm with a 1550 nm pump. Our measurements suggest the intermodal FWM is a viable means for large wavelength conversion and heralded photon sources.

We study the parametric amplification of electromagnetically induced transparency-assisted Rydberg six- and eight-wave mixing signals through a cascaded nonlinear optical process in a hot rubidium atomic ensemble both theoretically and experimentally. The shift of the resonant frequency (induced by the Rydberg–Rydberg interaction) of parametrically amplified six-wave mixing signal is observed. Moreover, the interplays between the dressing effects and Rydberg–Rydberg interactions in parametrically amplified multiwave mixing signals are investigated. The linear amplification of Rydberg multiwave mixing processes with multichannel nature acts against the suppression caused by Rydberg–Rydberg interaction and dressing effect.

The so-called “phase difference” is commonly introduced as a phenomenological parameter in Raman tensor theory, so as to fit the experimental data well. Although phase difference is widely recognized as an intrinsic property of crystals, its physics still remains ambiguous. Recently, Kranert et al. have presented a new formalism to explain the origin of phase difference theoretically. Here, we systematically conducted experimental research with polar phonons in wurtzite crystals, the results of which strongly suggest that the phase difference should be predetermined in a Raman tensor, rather than be treated as Raman tensor elements traditionally or as an intrinsic property. On the grounds of pinpointing existing logical flaws in Raman tensor study, we provide a logically clear paradigm.

Two-dimensional transition metal dichalcogenides are considered promising materials for next-generation photonics and nano-optical devices. Although many previous reports have shown saturable absorption of molybdenum diselenide (MoSe2), these nonlinear optical (NLO) properties of MoSe2 were measured in separate works and under different conditions with their hot-carrier relaxations. Here, we conducted a series of coherent studies on the NLO properties of few-layer MoSe2 via open-aperture Z-scan and degenerate pump-probe techniques. These measurements were taken to test the materials’ capabilities as a slow-saturable absorber. A slow-absorber model was employed to analyze the NLO measurements, and the results show that the NLO modulation depth was modeled to be 7.4% and 15.1% for the linear absorption coefficients of 5.22 cm 1 and 6.51 cm 1, respectively. The corresponding saturated intensities were modeled to be 39.37 MW/cm2 and 234.75 MW/cm2, respectively. The excitation carrier recovery time of few-layer MoSe2 was measured by degenerate pump-probe techniques to be ～220 ps. These nonlinear optical performances make it a promising slow-saturable absorber for passive mode locking in femtosecond lasers.

Microresonator-based Kerr frequency combs have attracted a great deal of attention in recent years, in which mode locking of the generated combs is associated with bright or dark cavity soliton formation. In this paper, we show that, different from soliton propagation along a waveguide, cavity solitons can be robustly formed under a unique dispersion profile with four zero-dispersion wavelengths. More importantly, such a dispersion profile exhibits much smaller overall dispersion, thus making it possible to greatly reduce the pump power by five to six times.

We report on infrared supercontinuum (SC) generation in step-index fluoroindate-based fiber by using an all-fiber laser source. In comparison to widely used ZBLAN fibers for high-power mid-infrared (MIR) SC generation, fluoroindate fibers have multiphoton absorption edges at significantly longer wavelengths and can sustain similar intensities. Recent developments highlighted in the present study allowed the production of fluoroindate fibers with MIR background loss of 2 dB/km, which is similar to or even better than ZBLAN fibers. By using an all-fiber picosecond laser source based on an erbium amplifier followed by a thulium power amplifier, we demonstrate the generation of 1.0 W infrared SC spanning over 2.25 octaves from 1 μm to 5 μm. The generated MIR SC also exhibits high spectral flatness with a 6 dB spectral bandwidth from 1.91 μm to 4.77 μm and an average power two orders of magnitude greater than in previous demonstrations with a similar spectral distribution.

High flatness, wide bandwidth, and high-coherence properties of supercontinuum (SC) generation in fibers are crucial in many applications. It is challenging to achieve SC spectra in a combination of the properties, since special dispersion profiles are required, especially when pump pulses with duration over 100 fs are employed. We propose an all-solid microstructured fiber composed only of hexagonal glass elements. The optimized fiber possesses an ultraflat all-normal dispersion profile, covering a wide wavelength interval of approximately 1.55 μm. An SC spectrum spanning from approximately 1030 to 2030 nm (corresponding to nearly one octave) with flatness <3 dB is numerically generated in the fiber with 200 fs pump pulses at 1.55 μm. The results indicate that the broadband ultraflat SC sources can be all-fiber and miniaturized due to commercially achievable 200-fs fiber lasers. Moreover, the SC pulses feature high coherence and a single pulse in the time domain, which can be compressed to 13.9-fs pulses with high quality even for simple linear chirp compensation. The Fourier-limited pulse duration of the spectrum is 3.19 fs, corresponding to only 0.62 optical cycles.

To achieve photon-pair generation scaling, we optimize the quality factor of microring resonators for efficient continuous-wave-pumped spontaneous four-wave mixing. Numerical studies indicate that a high intrinsic quality factor makes high pair rate and pair brightness possible, in which the maximums take place under overcoupling and critical-coupling conditions, respectively. We fabricate six all-pass-type microring resonator samples on a silicon-on-insulator chip involving gap width as the only degree of freedom. The signal count rate, pair brightness, and coincidence rate of all the samples are characterized, which are then compared with the modified simulations by taking the detector saturation and nonlinear loss into account. Being experimentally validated for the first time to the best of our knowledge, this work explicitly demonstrates that reducing the round-trip loss in a ring cavity and designing the corresponding optimized gap width are more effective to generate high-rate or high-brightness photon pairs than the conventional strategy of simply increasing the quality factor.

The pulse energy in the ultrafast soliton fiber laser oscillators is usually limited by the well-known wave-breaking phenomenon owing to the absence of a desirable real saturable absorber (SA) with high power tolerance and large modulation depth. Here, we report a type of microfiber-based MoTe2 SA fabricated by the magnetron-sputtering deposition (MSD) method. High-energy wave-breaking free soliton pulses were generated with pulse duration/pulse energy/average output power of 229 fs/2.14 nJ/57 mW in the 1.5 μm regime and 1.3 ps/13.8 nJ/212 mW in the 2 μm regime, respectively. To our knowledge, the generated soliton pulses at 1.5 μm had the shortest pulse duration and the highest output power among the reported erbium-doped fiber lasers mode locked by transition metal dichalcogenides. Moreover, this was the first demonstration of a MoTe2-based SA in fiber lasers in the 2 μm regime, and the pulse energy/output power are the highest in the reported thulium-doped fiber lasers mode locked by two-dimensional materials. Our results suggest that a microfiber-based MoTe2 SA could be used as an excellent photonic device for ultrafast pulse generation, and the MSD technique opens a promising route to produce a high-performance SA with high power tolerance and large modulation depth, which are beneficial for high-energy wave-breaking free pulse generation.

A spectrally flat mid-infrared supercontinuum (MIR-SC) spanning 2.8–3.9 μm with a maximum output power of 411 mW was generated in a holmium-doped ZBLAN fiber amplifier (HDZFA). A broadband fiber-based SC covering the 2.4–3.2 μm region was designed to seed the amplifier. Benefiting from the broadband seed laser, the obtained SC had a high spectral flatness of 3 dB over the range of 2.93–3.70 μm (770 nm). A spectral integral showed that the SC power beyond 3 μm was 372 mW, i.e., a power ratio of 90.6% of the total power. This paper, to the best of our knowledge, not only demonstrates the first spectrally flat MIR-SC directly generated in fluoride fiber amplifiers, but also reports the highest power ratio beyond 3 μm obtained in rare-earth-doped fluoride fiber until now.

We report an all-fiber, all-polarization maintaining (PM) source of widely tunable (1800–2000 nm) ultrashort pulses based on the amplification of coherent self-frequency-shifted solitons generated in a highly nonlinear fiber pumped with an Er-doped fiber laser. The system delivers sub-100 fs pulses with energies up to 8.6 nJ and is built entirely from PM optical fibers, without any free-space optics. The all-fiber alignment-free design significantly increases the suitability of such a source for field deployments.

Dual combs are an emerging tool to obtain unprecedented resolution, high sensitivity, ultrahigh accuracy, broad bandwidth, and ultrafast data updating rate in the fields of molecular spectroscopy, optical metrology, as well as optical frequency synthesis. The recent progress in chip-based microcombs has promoted the on-chip dual-comb measuring systems to a new phase attributed to the large frequency spacing and broad spectrum. In this paper, we demonstrate proof-of-concept dual-comb generation with orthogonal polarization in a single microresonator through pumping both the transverse-electric (TE) and transverse-magnetic (TM) modes simultaneously. The two orthogonal polarized pumps are self-oscillating in a fiber ring cavity. The generated dual comb exhibits excellent stability due to the intrinsic feedback mechanism of the self-locked scheme. The repetition rate of the two orthogonal combs is slightly different because of the mode spacing difference between the TE and TM modes. Such orthogonal polarized dual-combs could be a new comb source for out-of-lab applications in the fields of integrated spectroscopy, ranging measurement, optical frequency synthesis, and microwave comb generation.

We investigate frequency-comb generation in normal dispersion silicon microresonators from the near-infrared to mid-infrared wavelength range in the presence of multiphoton absorption and free-carrier effects. It is found that parametric oscillation is inhibited in the telecom wavelength range resulting from strong two-photon absorption. On the contrary, beyond the wavelength of 2200 nm, where three- and four-photon absorption are less detrimental, a comb can be generated with moderate pump power, or free-carriers are swept out by a positive-intrinsic-negative structure. In the temporal domain, the generated combs correspond to flat-top pulses, and the pulse duration can be easily controlled by varying the laser detuning. The reported comb generation process shows a high conversion efficiency compared with anomalous dispersion regime, which can guide and promote comb formation in materials with normal dispersion. As the comb spectra cover the mid-infrared wavelength range, they can find applications in comb-based radiofrequency photonic filters and mid-infrared spectroscopy.

We report on the enhancement of phase conjugation degenerate four-wave mixing (DFWM) in hot atomic Rb vapor by using a Bessel beam as the probe beam. The Bessel beam was generated using cross-phase modulation based on the thermal nonlinear optical effect. Our results demonstrated that the DFWM signal generated by the Bessel beam is about twice as large as that generated by the Gaussian beam, which can be attributed to the extended depth and tight focusing features of the Bessel beam. We also found that a DFWM signal with reasonable intensity can be detected even when the Bessel beam encounters an obstruction on its way, thanks to the self-healing property of the Bessel beam. This work not only indicates that DFWM using a Bessel beam would be of great potential in the fields of high-fidelity communication, adaptive optics, and so on, but also suggests that a Bessel beam would be of significance to enhance the nonlinear process, especially in thick and scattering media.

Oxygen-containing defects are very important for altering the nonlinear optical (NLO) properties of graphene. To investigate the correlation between oxygen-containing defects and the synergistic NLO response in graphene-based nanocomposites, we attached CdS nanocrystals on the surface of graphene (G) and prepared G/CdS nanohybrids (NHs) consisting of various oxygen-containing functional groups via a chemical method. The NLO absorption and refraction of G/CdS NHs under single pulse laser irradiation are enhanced by 10.8 times with the concentration decrease of surface oxygen-containing groups, which might be attributed to the local field effects and synergetic effects stemming from charge transfer between the two components. However, the optical nonlinearity is decreased with further concentration decrease, which might arise from sp2 fragment interconnection and surface defects in the NHs. The NLO absorption transformation from two-photon absorption to saturable absorption with oxygen decrease is observed, and intensity-related NLO absorption and refraction in NHs are also discussed. Meanwhile, the G/CdS NHs exhibit superior NLO properties, implying potential applications of NH material in NLO devices.

When a dielectric meta-atom is placed into a subwavelength metallic aperture, 20-fold enhanced electromagnetic transmission through the aperture is realized at the meta-atom’s resonant frequency. Additionally, when the incident electromagnetic power increases, thermal energy gathered by the meta-atom, which is converted from electromagnetic losses, can cause the meta-atom’s temperature to increase. Because of the high temperature coefficient of the meta-atom’s resonant frequency, this temperature increase causes a blueshift in the transmission peak. Therefore, this frequency-dependent enhanced electromagnetic transmission even produces a nonlinear effect at low incident powers. Over an incident power range from 0 to 20 dBm, measured and simulated spectra near the meta-atom’s resonant frequency show distinctly nonlinear transmission.

As a kind of two-dimensional transition metal dichalcogenide material, tungsten diselenide (WSe2) has attracted increasing attention, owing to its gapped electronic structure, relatively high carrier mobility, and valley pseudospin, all of which show its valuable nonlinear optical properties. There are few studies on the nonlinear optical properties of WSe2 and correlation with its electronic structure. In this paper, the effects of spatial self-phase modulation (SSPM) and distortion influence of WSe2 ethanol suspensions are systematically studied, namely, the nonlinear refractive index and third-order nonlinear optical effect. We obtained the WSe2 dispersions SSPM distortion formation mechanism, and through it, we calculated the nonlinear refractive index n2, nonlinear susceptibility χ(3), and their wavelength dependence under the excitation of 457 nm, 532 nm, and 671 nm lasers. Moreover, by use of its strong and broadband nonlinear optical response, all-optical switching of two different laser beams due to spatial cross-phase modulation has been realized experimentally. Our results are useful for future optical devices, such as all-optical switching and all-optical information conversion.

We have studied the two- and three-photon absorption (2PA and 3PA) properties of Mn-doped CsPbCl3 two-dimensional nanoplatelets (2D NPs) and cubic nanocrystals. Compared with their cubic counterparts, the Mn-doped 2D NPs exhibit stronger quantum confinement effects that can more efficiently enhance their dopant-carrier exchange interactions and multiphoton absorption. More specifically, the maximum volume-normalized 2PA and 3PA cross sections of the 2D NPs were 6.8 and 7.2 times greater than those of their cubic counterparts, respectively, reaching up to 1237 GM/nm3 in the visible light band and 2.24×10 78 cm6·s2·photon 2/nm3 in the second biological window, respectively.

We systematically investigate the influences of the input infrared spectrum, chirp, and polarization on the emitted intense terahertz spectrum and spatial dispersion in lithium niobate via optical rectification. The terahertz yield and emission spectrum depend on both the chirp and spectrum of the input pump laser pulses. We also observe slight non-uniform spatial dispersion using a knife-edge measurement, which agrees well with the original predictions. The possible mechanism is the nonlinear distortion effect caused by high-energy laser pumping. Our study is very important and useful for developing intense terahertz systems with applications in extreme terahertz sciences and nonlinear phenomena.

Future quantum information networks operated on telecom channels require qubit transfer between different wavelengths while preserving quantum coherence and entanglement. Qubit transfer is a nonlinear optical process, but currently the types of atoms used for quantum information processing and storage are limited by the narrow bandwidth of upconversion available. Here we present the first experimental demonstration of broadband and high-efficiency quasi-phase matching second-harmonic generation (SHG) in a chip-scale periodically poled lithium niobate thin film. We achieve a large bandwidth of up to 2 THz for SHG by satisfying quasi-phase matching and group-velocity matching simultaneously. Furthermore, by changing the film thickness, the central wavelength of the quasi-phase matching SHG bandwidth can be modulated from 2.70 μm to 1.44 μm. The reconfigurable quasi-phase matching lithium niobate thin film provides a significant on-chip integrated platform for photonics and quantum optics.

Microcomb generation with simultaneous χ(2) and χ(3) nonlinearities brings new possibilities for ultrabroadband and potentially self-referenced integrated comb sources. However, the evolution of the intracavity field involving multiple nonlinear processes shows complex dynamics that are still poorly understood. Here, we report on strong soliton regulation induced by fundamental–second-harmonic (FD-SH) mode coupling. The formation of solitons from chaos is extensively investigated based on coupled Lugiato–Lefever equations. The soliton generation shows more deterministic behaviors in the presence of FD-SH mode interaction, which is in sharp contrast with the usual cases where the soliton number and relative locations are stochastic. Deterministic single soliton transition, soliton binding, and prohibition are observed, depending on the phase-matching condition and coupling coefficient between the fundamental and second-harmonic waves. Our finding provides important new insights into the soliton dynamics in microcavities with simultaneous χ(2) and χ(3) nonlinearities and can be immediate guidance for broadband soliton comb generation with such platforms.

An overview of the progress on pulse-preserving, coherent, nonlinear fiber-based supercontinuum generation is presented. The context encompasses various wavelength ranges and pump sources, starting with silica photonic crystal fibers pumped with 1.0 μm femtosecond lasers up to chalcogenide step-index and microstructured fibers pumped from optical parametric amplifiers tuned to mid-infrared wavelengths. In particular, silica and silicate-based all-normal dispersion (ANDi) photonic crystal fibers have been demonstrated for pumping with femtosecond lasers operating at 1.56 μm with the recorded spectra covering 0.9–2.3 μm. This matches amplification bands of robust fiber amplifiers and femtosecond lasers. The review therefore focuses specifically on this wavelength range, discussing glass and nonlinear fiber designs, experimental results on supercontinuum generation up to the fundamental limit of oxide glass fiber transmission around 2.8 μm, and various limitations of supercontinuum bandwidth and coherence. Specifically, the role of nonlinear response against the role of dispersion profile shape is analyzed for two different soft glass ANDi fibers pumped at more than 2.0 μm. A spatio-temporal interaction of the fundamental fiber mode with modes propagating in the photonic lattice of the discussed ANDi fibers is shown to have positive effects on the coherence of the supercontinuum at pump pulse durations of 400 fs. Finally, the design and development of graded-index, nanostructured core optical fibers are discussed. In such structures the arbitrary shaping of the core refractive index profile could significantly improve the engineering flexibility of dispersion and effective mode area characteristics, and would be an interesting platform to further study the intermodal interaction mechanisms and their impact on supercontinuum coherence for sub-picosecond laser pumped setups.

An opposite-chirped frequency-domain optical parametric amplification (OC-FOPA) design is demonstrated and numerically verified. This scheme combines both an ultrabroad seeding generation and the subsequent effective amplification in one single optical parametric amplification stage. Based on a slightly asymmetrical 4-f optical system, the spectral contents of both pump and signal waves are spectrally dispersed with opposite spatial chirps, to broaden the initial idler seeding. Via a properly designed fan-out periodically poled LiNbO3 chip, nearly perfect quasi phase matching can be realized across the full spectrum, whereby each individual spectral pair precisely maps to its required grating period. Full-dimensional simulations based on commercial ～110 fs (FWHM) near-infrared (near-IR) lasers at 790 and 1030 nm are quantitatively discussed, and few-cycle mid-IR laser pulses (～60 fs at 3.4 μm) plus a high conversion efficiency exceeding 50% are theoretically predicted. By means of a high-power pump source, the OC-FOPA scheme can be also applied to directly produce high-intensity carrier-envelope-phase-stabilized mid-IR idler pulses.

The scattering matrix theory has been developed to calculate the third-order nonlinear effect in sphere-graphene-slab structures. By designing structural parameters, we have demonstrated that the incident electromagnetic wave can be well confined in the graphene in these structures due to the formation of a bound state in the continuum (BIC) of radiation modes. Based on such a bound state, third-harmonic (TH) generation and four-wave mixing (FWM) have been studied. It is found that the efficiency of TH generation in monolayer graphene can be enhanced about 7 orders of magnitude. It is interesting that we can design structure parameters to make all beams (the pump beam, probe beam, and generated FWM signal) be BICs at the same time. In such a case, the efficiency of FWM in monolayer graphene can be enhanced about 9 orders of magnitude. Both the TH and FWM signals are sensitive to the wavelength, and possess high Q factors, which exhibit very good monochromaticity. By taking suitable BICs, the selective generation of TH and FWM signals for S- and P-polarized waves can also be realized, which is beneficial for the design of optical devices.

We report the first observation, to the best of our knowledge, of sum-frequency generation in on-chip lithium niobate microdisk resonators. The sum-frequency signal in the 780 nm band, distinct in wavelength from second-harmonic signals, was obtained in lithium niobate microresonators under the pump of two individual 1550 nm band lasers. The sum-frequency conversion efficiency was measured to be 1.4×10?7 mW?1. The dependence of the intensities of the nonlinear signals on the total pump power and the wavelength of one pump laser was investigated while fixing the wavelength of the other. This work paves the way for applications of on-chip lithium niobate microdisk resonators ranging from infrared single-photon detection to infrared spectroscopy.

The pulse dynamics of harmonic mode-locking in a dissipative soliton resonance (DSR) region in an erbium-doped fiber ring laser is investigated at different values of anomalous dispersion. The fiber laser is mode-locked by a nonlinear polarization rotation technique. By inserting 0–200 m anomalous dispersion single-mode fiber in the laser cavity, the cavity length is changed from 17.3 to 217.3 m, and the corresponding dispersion of the cavity ranges from ?0.27 to ?4.67 ps2. The observed results show that the tuning range of repetition rate under a harmonic DSR condition is highly influenced by the cavity dispersion. Furthermore, it is found that, by automatically adjusting their harmonic orders, the lasers can work at certain values of repetition rate, which are independent of the cavity length and dispersion. The pulses at the same repetition rate in different laser configurations have similar properties, demonstrating that each achievable repetition rate represents an operation regime of harmonic DSR lasers.

Octave-spanning frequency comb generation in microresonators is promising, but strong spectral losses caused by material absorption and mode coupling between two polarizations or mode families can be detrimental. We examine the impact of the spectral loss and propose robust comb generation with a loss of even 300 dB/cm. Cavity nonlinear dynamics show that a phase change associated with spectral losses can facilitate phase matching and Kerr comb generation. Given this unique capability, we propose a novel architecture of on-chip spectroscopy systems.

This work presents the saturable absorption (SA) properties of CsPbBr3 perovskite quantum dots (QDs). The perovskite QDs show excellent SA performance with a nonlinear absorption coefficient of ?35×10?2 cm/GW and a figure of merit of 3.7×10?14 esu?cm. Further, their use as saturable absorbers in a passively Q-switched visible solid-state laser for the generation of soliton pulses is demonstrated. These results demonstrate the potential for the perovskite QDs to act as saturable absorbers.

We report the investigation on the performance of an amplification assisted difference frequency generation (AA-DFG) system driven by pulsed pump and continuous-wave primary signal lasers. A monolithic tandem lithium niobate superlattice was employed as the nonlinear crystal with a uniform grating section for the DFG process, followed by a chirp section for the optical parametric amplification process. The impacts of pump pulse shape, primary signal power, input beam diameter, and crystal structure on the pump-to-idler conversion efficiency of the AA-DFG system were comprehensively studied by numerically solving the coupled wave equations. It is concluded that square pump pulse and high primary signal power are beneficial to high pump-to-idler conversion efficiency. In addition, tighter input beam focus and smaller DFG length proportion could redeem the reduction in conversion efficiency resulting from wider acceptance bandwidths for the input lasers. We believe that such systems combining the merits of high stability inherited from cavity-free configuration and high efficiency attributed from the cascaded nonlinear conversion should be of great interest to a wide community, especially when the pulse shaping technique is incorporated.

We experimentally demonstrate the nonlinear interaction between two chirped broadband single-photon-level coherent states. Each chirped coherent state is generated in independent fiber Bragg gratings. They are simultaneously coupled into a high-efficiency nonlinear waveguide, where they are converted into a narrowband single-photon state with a new frequency by the process of sum-frequency generation (SFG). A higher SFG efficiency of 1.06×10 7 is realized, and this efficiency may achieve heralding entanglement at a distance. This also made it possible to realize long-distance quantum communication, such as device-independent quantum key distribution, by directly using broadband single photons without filtering.

Two-dimensional (2D) periodical Au and indium tin oxide (ITO) nanocomposite arrays have been fabricated based on a self-assembled nanosphere lithography technique. A button-shaped Au nanoparticle was formed on each hollow hemisphere-shaped ITO shell. Importantly, the underlying formation mechanism during the thermal treatment has been thoroughly explored by comparing structures resulting from different deposition conditions in detail. Compared to the Au nanoparticle arrays without ITO shells, the Au/ITO nanocomposite arrays showed a stronger localized surface plasmon resonance effect and higher absorption in the near-infrared (NIR) region, benefiting from the free-electron interaction enhancement between Au and ITO. The nonlinear optical properties were investigated using a modified femtosecond intensity-scan system, and the results demonstrated Au/ITO nanocomposite arrays with a remarkable two-photon absorption saturation effect for femtosecond pulses at 1030 nm. The versatile NIR optical responses indicate the great potential of the elaborately prepared 2D periodical Au/ITO nanocomposite arrays in many applications such as solar cells, photocatalysis, and novel nano optoelectronic devices.

The spectral purity of fiber lasers has become a critical issue in both optical sensing and communication fields. As a result of ultra-narrow intrinsic linewidth, stimulated thermal Rayleigh scattering (STRS) has presented special potential to compress the linewidth of fiber lasers. To suppress stimulated Brillouin scattering (SBS), the most dominant disturbance for STRS in optical fibers, a semi-quantitative estimation has been established to illuminate the mechanism of suppressing SBS in a periodic tapered fiber, and it agrees with experimental results. Finally, a linewidth compression device based on STRS is integrated into a single-longitudinal-mode ring-cavity fiber laser with secondary cavities, and its linewidth is verified to be 200 Hz through a self-heterodyne detecting and Voigt fitting method.

Dual-pumped microring-resonator-based optical frequency combs (OFCs) and their temporal characteristics are numerically investigated and experimentally explored. The calculation results obtained by solving the driven and damped nonlinear Schr dinger equation indicate that an ultralow coupled pump power is required to excite the primary comb modes through a non-degenerate four-wave-mixing (FWM) process and, when the pump power is boosted, both the comb mode intensities and spectral bandwidths increase. At low pump powers, the field intensity profile exhibits a cosine variation manner with frequency equal to the separation of the two pumps, while a roll Turing pattern is formed resulting from the increased comb mode intensities and spectral bandwidths at high pump powers. Meanwhile, we found that the power difference between the two pump fields can be transferred to the newly generated comb modes, which are located on both sides of the pump modes, through a cascaded FWM process. Experimentally, the dual-pumped OFCs were realized by coupling two self-oscillating pump fields into a microring resonator. The numerically calculated comb spectrum is verified by generating an OFC with 2.0 THz mode spacing over 160 nm bandwidth. In addition, the formation of a roll Turing pattern at high pump powers is inferred from the measured autocorrelation trace of a 10 free spectral range (FSR) OFC. The experimental observations accord well with the numerical predictions. Due to their large and tunable mode spacing, robustness, and flexibility, the proposed dual-pumped OFCs could find potential applications in a wide range of fields, including arbitrary optical waveform generation, high-capacity optical communications, and signal-processing systems.

We report on the modeling, simulation, and experimental demonstration of complete mode crossings of Fano resonances within chip-integrated microresonators. The continuous reshaping of resonant line shapes is achieved via nonlinear thermo-optical tuning when the cavity-coupled optical pump is partially absorbed by the material. The locally generated heat then produces a thermal field, which influences the spatially overlapping optical modes, allowing us to alter the relative spectral separation of resonances. Furthermore, we exploit such tunability to continuously probe the coupling between different families of quasi-degenerate modes that exhibit asymmetric Fano interactions. As a particular case, we demonstrate a complete disappearance of one of the modal features in the transmission spectrum as predicted by Fano [Phys. Rev.124, 1866 (1961)PHRVAO0031-899X10.1103/PhysRev.124.1866]. The phenomenon is modeled as a third-order nonlinearity with a spatial distribution that depends on the stored optical field and thermal diffusion within the resonator. The performed nonlinear numerical simulations are in excellent agreement with the experimental results, which confirm the validity of the developed theory.

We have demonstrated a high-average-power, high-repetition-rate optical terahertz (THz) source based on difference frequency generation (DFG) in the GaSe crystal by using a near-degenerate 2 μm intracavity KTP optical parametric oscillator as the pump source. The power of the 2 μm dual-wavelength laser was up to 12.33 W with continuous tuning ranges of 1988.0–2196.2 nm/2278.4–2065.6 nm for two waves. Different GaSe cystal lengths have been experimentally investigated for the DFG THz source in order to optimize the THz output power, which was in good agreement with the theoretical analysis. Based on an 8 mm long GaSe crystal, the THz wave was continuously tuned from 0.21 to 3 THz. The maximum THz average power of 1.66 μW was obtained at repetition rate of 10 kHz under 1.48 THz. The single pulse energy amounted to 166 pJ and the conversion efficiency from 2 μm laser to THz output was 1.68×10 6. The signal-to-noise ratio of the detected THz voltage was 23 dB. The acceptance angle of DFG in the GaSe crystal was measured to be 0.16°.

Transverse mode instability (TMI) has become the major limitation for power scaling of fiber lasers with nearly diffraction-limited beam quality. Compared with a co-pumped fiber laser, a counter-pumped fiber laser reveals TMI threshold enhancement through a semi-analytical model calculation. We demonstrated a 2 kW high-power counter-pumped all-fiberized laser without observation of TMI. Compared with the co-pumped scheme, the TMI threshold is enhanced at least 50% in counter-pumped scheme, moreover, stimulated Raman scattering and four-wave mixing are suppressed simultaneously.

A mode-locked thulium-doped fiber laser (TDFL) based on nonlinear polarization rotation (NPR) with different net anomalous dispersion is demonstrated. When the cavity dispersion is ?1.425 ps2, the noise-like (NL) pulse with coherence spike width of 406 fs and pulse energy of 12.342 nJ is generated at a center wavelength of 2003.2 nm with 3 dB spectral bandwidth of 23.20 nm. In the experimental period of 400 min, the 3 dB spectral bandwidth variation, the output power fluctuation, and the central wavelength shift are less than 0.06 nm, 0.04 dB, and 0.4 nm, respectively, indicating that the NPR-based TDFL operating in the NL regime holds good long-term stability.

We experimentally investigated the nonlinear optical response in few-layer oxidized black phosphorus (OBP) by the femtosecond Z-scan measurement technique, and found that OBP not only possesses strong ultrafast saturable absorption but also a nonlinear self-defocusing effect that is absent in black phosphorus (BP). The saturable absorption property originates mainly from the direct band structure, which is still maintained in OBP. The emergence of self-defocusing might originate from the combined consequences of the oxygen-induced defects in BP. Our experimental findings might constitute the first experimental evidence on how to dynamically tuneits nonlinear property, offering an inroad in tailoring its optical properties through chemical modification (oxidation, introducing defects, etc.). The versatile ultrafast nonlinear optical properties (saturable absorption and self-defocusing) imply a significant potential of the layered OBP in the development of unprecedentedoptoelectronic devices, such as mode lockers, optical switches, laser beam shapers, and wavelength converters.China Postdoctoral Science Foundation (2015M580731); Science and Technology Planning Project of Guangdong Province (2016B050501005).

We investigate in this paper the influence of slow light on the balance between the Kerr and two-photon absorption (TPA) processes in silicon slotted hybrid nonlinear waveguides. Three typical silicon photonic waveguide geometries are studied to estimate the influence of the light slow-down factor on the mode field overlap with the silicon region, as well as on the complex effective nonlinear susceptibility. It is found that slotted photonic crystal modes tend to focalize in their hollow core with increasing group index (nG) values. Considering a hybrid integration of nonlinear polymers in such slotted waveguides, a relative decrease of the TPA process by more factor of 2 is predicted from nG
10 to nG
50. As a whole, this work shows that the relative influence of TPA decreases for slotted waveguides operating in the slow light regime, making them a suitable platform for third-order nonlinear optics.

All-optical two-channel format conversion is proposed and experimentally demonstrated from a 40 Gbit/s polarization multiplexing (Pol-MUX) non-return-to-zero quadrature phase-shift keying (QPSK) signal to Pol-MUX binary phase-shift keying (BPSK) signals by using phase-doubled four-wave mixing effects with two polarization-angled pumps in a silicon waveguide. The eye diagrams and constellation diagrams of the original QPSK sequences and the converted BPSK sequences of each channel are clearly observed on the two polarization states. Moreover, the bit error rates (BERs) of the two converted idlers are measured. The power penalties of all these converted BPSK sequences on both X and Y polarization states are less than 3.4 dB at a BER of 3.8 × 10?3.(20130101110089); Natural Science Foundation of Zhejiang Province (LY14F050006).

We study a nonlinear lossless polarizer (NLP), a fiber-based device able to control the polarization of an optical signal while preserving its energy. The NLP exploits the lossless polarization attraction (LPA) generated by the Kerr interactions between the signal and a fully polarized continuous wave (CW) pump. By employing a copropagating pump, we show that the effectiveness of LPA depends on the joint action of the Kerr nonlinearity and the mutual delay between signal and pump. We find the optimal pump wavelength placement and demonstrate that true LPA occurs only within a limited range of delay values. Thus, we explain why the copropagating NLP is more flexible and power efficient compared with the traditional counterpropagating NLP.

Gapless linear energy dispersion of graphene endows it with unique nonlinear optical properties, including broadband nonlinear absorption and giant nonlinear refractive index. Herein, we experimentally observed that fewlayers graphene has obvious nonlinear absorption and large nonlinear refraction, as investigated by the Z-scan technique in the mid-infrared (mid-IR) regime. Our study may not only, for the first time to our knowledge, verify the giant nonlinear refractive index of graphene (～10?7 cm2∕W) at the mid-IR, which is 7 orders of magnitude larger than other conventional bulk materials, but also provide some new insights for graphene-based mid-IR photonics, potentially leading to the emergence of several new conceptual mid-IR optoelectronics devices.

The generation of multicolored sidebands with the spectrum from 377 to 970 nm in a 0.5-mm-thick N-WG280 Schott glass based on a cascaded four-wave mixing (CFWM) process is demonstrated. The experimental setup is compact and economical. A pulse with a broadened spectrum from 670 to 900 nm is generated by utilizing two 0.18-mm-thick fused silica glass plates and is used to provide two input beams for the CFWM process. The new frequency components generated from the self-phase modulation effect in the two thin glass plates contribute to the broadening of the total spectral range of the generated multicolored sidebands.

A quasi-two-dimensional layer of MoS2 was placed on top of a silicon optical waveguide to form a MoS2–silicon hybrid structure. Chirped pulse self-phase modulation measurements were carried out to determine the optical Kerr nonlinearity of the structure. The observed increase in the spectral broadening of the optical pulses in the MoS2–silicon waveguide compared with the silicon waveguides indicated that the third-order nonlinear effect in MoS2 is about 2 orders of magnitude larger than that in silicon. The measurements show that MoS2 has an effective optical Kerr coefficient of about 1.1 × 10?16 m2∕W. This work reveals the potential application of MoS2 to enhance the nonlinearity of hybrid silicon optical devices.

We proposed a new scheme of controlling second-harmonic generation by enhanced Kerr electro-optic nonlinearity. We designed a structure that can implement the cascaded Pockels effect and second-harmonic generation simultaneously. The energy coupling between the fundamental lights of different polarizations led to a large nonlinear phase shift and, thus, an effective electro-optic nonlinear refractive index. The effective nonlinearity can be either positive or negative, causing the second-harmonic spectra to move toward the coupling center, which, in turn, offered us a way to measure the effective electro-optic nonlinear refractive index. The corresponding enhanced Kerr electro-optic nonlinearity is more than three orders of magnitude higher than the intrinsic value. These results open a door to manipulate the nonlinear phase by applying an external electric field instead of light intensity in noncentrosymmetric crystals.

All-optical canonical logic units at 40 Gb/s using bidirectional four-wave mixing (FWM) in highly nonlinear fiber are proposed and experimentally demonstrated. Clear temporal waveforms and correct pattern streams are successfully observed in the experiment. This scheme can reduce the amount of nonlinear devices and enlarge the computing capacity compared with general ones. The numerical simulations are made to analyze the relationship between the FWM efficiency and the position of two interactional signals.

Using a strong nonlinear saturation absorption effect is one technique for breaking through the diffraction limit. In this technique, formation of a dynamic and reversible optical pinhole channel and transient superresolution is critical. In this work, a pump–probe transient detection and observation–experimental setup is constructed to explore the formation process directly. A Ge2Sb2Te5 thin film with strong nonlinear saturation absorption is investigated. The dynamic evolution of the optical pinhole channel is detected and imaged, and the transient superresolution spot is directly captured experimentally. Results verify that the superresolution effect originates from the generation of an optical pinhole channel and that the formation of the optical pinhole channel is dynamic and reversible. A good method is provided for direct detection and observation of the transient process of the superresolution effect of nonlinear thin films.

A novel method for converting an array of out-of-phase lasers into one of in-phase lasers that can be tightly focused is presented. The method exploits second-harmonic generation and can be adapted for different laser arrays geometries. Experimental and calculated results, presented for negatively coupled lasers formed in a square, honeycomb, and triangular geometries are in good agreement.

The dynamic characteristics are investigated for a microring laser with an external radius of 12 μm subject to external optical injection. Single-mode operation with a side mode suppression ratio of 33.4 dB is realized at a biasing current of 25 mA and a temperature of 290 K, and the corresponding small-signal modulation response is obtained with a resonance peak frequency of 7.5 GHz. Under the optical injection from a tunable laser, the improvements of the small-signal modulation response induced by four-wave mixing are observed for the microring laser, which shows an additional resonance peak around the frequency of the beat frequency between the lasing mode and the injecting light. Furthermore, optical generation of a microwave signal is realized by the light beating between the lasing mode and the injecting light measured by a high-speed photodetector and a spectrum analyzer.

With the development of semiconductor technology, semiconductor laser devices and semiconductor laser pump solid-state laser devices have been widely applied in z-scan experiments. However, the feedback light-induced output instability of semiconductor laser devices can negatively affect the accurate testing of the nonlinear index. In this work, the influence of feedback light on z-scan measurement is analyzed. Then the calculated formula of feedback light-induced false nonlinear z-scan curves is theoretically derived and experimentally verified. Two methods are proposed to reduce or eliminate the feedback light-induced false nonlinear effect. One is the addition of an attenuator to the z-scan optical path, and the other is the addition of an opto-isolator unit to the z-scan setup. The experimental and theoretical results indicate that the feedback light-induced false nonlinear effect is markedly reduced and can even be ignored if appropriate parameters are chosen. Thus, theoretical and experimental methods of eliminating the negative effect of feedback light on z-scan measurement are useful for accurately obtaining the nonlinear index of a sample.

We present imaging experiments in focusing Kerr media using digital holography and digital reverse propagation (DRP) of the wave. For moderate power, the nonlinear DRP algorithm can be used to improve the quality of images over the linear DRP. We discuss the limits of the method at high power, the role of small-scale filaments, and the problem of time-dependent self-phase modulation.

The factors that influence the generation of a high-quality optical frequency comb (OFC) based on a recirculating frequency shifter (RFS) due to the maximum output power and noise figure of Er-doped fiber amplifier (EDFA) are studied theoretically and experimentally. Based on the theoretical analysis, numerical simulations and experiments under different EDFA parameters have been carried out. The results show that the performance of the OFC based on a RFS can be improved effectively by optimizing the maximum output power and the noise figure of the EDFA.